整体式结构化催化剂与反应器适用于气液固多相催化等反应，已成为一种过程强化的高效反应器。针对化学工业中一大类受传递控制的气液固三相催化反应（如苯与烯烃烷基化、蒽醌加氢制取过氧化氢等），采用数学模型与实验研究（包括冷模和热态）相结合的方法，① 研究蜂窝整体体式结构化催化剂与反应器从催化剂原粉到载体涂层的制备技术及其表界面调控机制；② 研究蜂窝整体式结构化催化剂与反应器连同相应的气液预分布器一起构成的气液固三相催化反应的数学模型，放大策略是CFD模型 + 混合池模型 + CFD模型，提出新型、有效的气液预分布器结构，形成过程强化成套技术；③ 面向石油化工中常见而重要的苯与丙烯烷基化合成异丙苯体系，确定可行操作域及最优的结构参数和操作参数，为这类高效反应器的大规模工业化提供基础研究数据和可行性分析。

Structured catalysts and reactors are suitable for gas-liquid-solid three-phase catalytic reaction systems, and have been becoming high-efficiency reactors for process intensification (PI). As we know, in chemical industry there exist a typical class of mass transfer-limiting gas-liquid-solid catalytic reactions (e.g., alkylation of benzene with olefins, and the synthesis of hydrogen peroxide by the anthraquinone method). For these reaction systems, we focus on i) studying the catalyst preparation technology from powder to washcoating on substrates as well as the surface/interface regulation mechanism; ii) studying the mathematical modeling of gas-liquid-solid catalytic reactions together with a gas-liquid pre-distributor, the scale-up strategy being the combination of CFD (computational fluid dynamics) + mixing pool model + CFD. Meanwhile, a new-type pre-distributor will be designed, thus forming a complete PI technology; and iii) determining the feasible operating regions and optimum structural and operating parameters, aiming at the alkylation of benzene with propylene to produce cumene which is a common and important reaction system in petrochemical industry. This project will provide the basic data and feasible analysis for the actual industrial applications of structured catalysts and reactors.