微通道内卫星液滴生成—惯性分离一体化原理及并行放大准则

批准号:
21878212
项目类别:
面上项目
资助金额:
66.0 万元
负责人:
付涛涛
依托单位:
学科分类:
B0802.传递过程
结题年份:
2022
批准年份:
2018
项目状态:
已结题
项目参与者:
刘偲、张沁丹、郭戎威、张翀、马蕊、杨潇寒、沈秋颖、徐子懿、米晟
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中文摘要
由于非线性动态特征,液液界面破裂过程常伴随卫星液滴的产生,对基于液滴的微流体技术均一性和精准化目标提出了挑战。本项目针对微流体界面失稳复杂动力学特征,阐释卫星液滴的生成机制。结合惯性微流体新概念,探究卫星液滴的惯性分离机制。提出卫星液滴生成—惯性微流体分离一体化方法,并构建相应过程的并行放大准则。基于界面动力学、自相似性原理、惯性微流体基本原理、并行微通道数目放大准则,采用高速摄像仪、微粒子图像测速仪等先进测量手段,结合耗散粒子动力学及流体体积法等模拟方法,考察微通道构型与尺寸、流体流量、流体物性如黏度及流变性、表面张力及表面活性剂浓度等对卫星液滴生成、惯性分离及生成—惯性分离微流体并行放大过程的影响,构建相应过程的预测模型和调控准则。本项目的实施,有利于实现微流体技术生产单分散性液滴的精准化目标,为微流体与复杂流体相关的界面动力学行为与调控夯实基础。
英文摘要
Due to the nonlinear dynamics, the rupture process of liquid-liquid interface often accompanies the production of satellite droplets, which challenges the uniformity and precision of droplet-based microfluidics technology. In this project, the mechanism of satellite droplet formation is revealed, according to the complex dynamics of interfacial instability in microfluidics. Based on the new concept of the inertial microfluidics, the mechanism of the separation of satellite droplet by using the inertial microfluidics is highlighted. The integration principle of generation – inertial microfluidics separation for the satellite droplet is proposed, as well as the parallelization criterion for the corresponding numbering-up. Based on the principle of interfacial dynamics, self-similarity, inertial microfluidics and numbering-up strategy of parallelized microchannels, the advanced measurement methods such as high-speed camera and micro-particle image velocimetry, combined with the dissipative particle dynamics and volume of fluids method, the influences of the configuration and size of microchannel, flow rate of fluid, physical properties of fluid such as viscosity and rheology, surface tension and surfactant concentration on the generation process, inertial separation and microfluidic parallelization during the numbering-up of integrated generation-inertial separation for satellite droplet are studied, and the predictive model and manipulation rule of the corresponding process are constructed. The implementation of this project is beneficial to realize the target of precision in producing monodisperse droplets with microfluidics technology, and to lay a solid foundation for the interfacial dynamics and regulation of microfluidics and complex fluids.
由于非线性动态特征,液液界面破裂过程常伴随卫星液滴的产生,对基于液滴的微流体技术均一性和精准化目标提出了挑战。本项目针对微流体界面失稳复杂动力学特征,阐释卫星液滴的生成机制。结合惯性微流体新概念,探究卫星液滴的惯性分离机制。提出卫星液滴生成—惯性微流体分离一体化方法,并构建相应过程的并行放大准则。本项目采用可视化实验、模拟及理论分析相结合的方法,探究了微通道内牛顿/非牛顿流体液液两相流及卫星液滴的生成调控、惯性分离及微通道的并行化数目放大机制。主要研究内容及结果为:1)探明了不同构型微通道中牛顿及非牛顿流体液滴生成时界面动态演化规律;2)阐明了卫星液滴生成机理及动力学机制,并提出了相应的调控方法;3)针对不同构型的微通道提出了并行放大及制备均一性液滴的指导性准则,构建了相应过程的预测模型。基于相关成果,发表了国内外学术论文18篇,其中SCI论文12篇,AIChE J 2篇、CES 2篇、《化工学报》6篇。参加了国内外学术会议9人次。培养了博士生1名,硕士生8名。本项目的实施,将为微流体与复杂流体相关的界面动力学行为及调控奠定良好的基础,为基于液滴的微流体技术的精确性和精准化发展夯实坚实的理论基础。
期刊论文列表
专著列表
科研奖励列表
会议论文列表
专利列表
Effects of the resultant force due to two-phase density difference on droplet formation in a step-emulsification microfluidic device
阶梯乳化微流控装置中两相密度差合力对液滴形成的影响
DOI:10.1016/j.jiec.2022.03.029
发表时间:2022-03
期刊:Journal of Industrial and Engineering Chemistry
影响因子:6.1
作者:Zhiwei Zhang;Mengyu Fan;Qianqiao Wang;Huaiyu Li;Chunying Zhu;Youguang Ma;Taotao Fu
通讯作者:Taotao Fu
Pressure drop of single phase flow in microchannels and its application in characterizing the apparent rheological property of fluids
微通道内单相流压降及其在表征流体表观流变特性中的应用
DOI:10.1007/s10404-019-2241-y
发表时间:2019
期刊:Microfluidics and Nanofluidics
影响因子:2.8
作者:Yang Xiaohan;Weldetsadik Netsanet Tesfaye;Hayat Zafar;Fu Taotao;Jiang Shaokun;Zhu Chunying;Ma Youguang
通讯作者:Ma Youguang
DOI:10.1002/aic.17780
发表时间:2022-05
期刊:AIChE Journal
影响因子:3.7
作者:Xiyang Liu;Shaokun Jiang;Chunying Zhu;Youguang Ma;Taotao Fu
通讯作者:Taotao Fu
Deformation and breakup of droplets in a double T-junction microdisperser with double input of the continuous phase
双输入连续相的双 T 形连接微分散器中液滴的变形和破碎
DOI:10.1016/j.cep.2021.108674
发表时间:2022
期刊:Chemical Engineering and Processing - Process Intensification
影响因子:--
作者:Langyu Liu;Cong Duan;Shaokun Jiang;Chunying Zhu;Youguang Ma;Taotao Fu
通讯作者:Taotao Fu
Early stage of externally driven filling of viscous fluids within a microfluidic pore-doublet network
微流体双孔网络内粘性流体的外部驱动填充的早期阶段
DOI:10.1063/5.0077697
发表时间:2022-02
期刊:Physics of Fluids
影响因子:4.6
作者:Cong Duan;Xiaohan Yang;Shaokun Jiang;Chunying Zhu;Youguang Ma;Taotao Fu
通讯作者:Taotao Fu
复杂流体液液两相流微化工的放大机制及界面效应
- 批准号:22378295
- 项目类别:面上项目
- 资助金额:50万元
- 批准年份:2023
- 负责人:付涛涛
- 依托单位:
高黏/非牛顿流体气液微反应器并行微通道内气泡群非均匀结构介尺度动力学
- 批准号:91634105
- 项目类别:重大研究计划
- 资助金额:67.0万元
- 批准年份:2016
- 负责人:付涛涛
- 依托单位:
微通道内气泡聚并、破裂过程的界面演化规律及界面传质机理
- 批准号:21106093
- 项目类别:青年科学基金项目
- 资助金额:25.0万元
- 批准年份:2011
- 负责人:付涛涛
- 依托单位:
国内基金
海外基金
