The enhanced photocatalytic reduction of uranium(VI) by ZnS@g-C3N4 heterojunctions under sunlight

The enhanced photocatalytic reduction of uranium(VI) by ZnS@g-C3N4 heterojunctions under sunlight
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ZnS@g-C3N4异质结在阳光下增强光催化还原铀(VI)

DOI:
10.1007/s10967-021-07784-y
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发表时间:
2021-06
影响因子:
1.6
通讯作者:
Yunhai Liu
Yunhai Liu
中科院分区:
化学4区
文献类型:
--
作者:
Fan Wu;Zhibin Zhang;Zhongping Cheng;Runze Zhou;Yuling Lin;Yuhui Liu;Youqun Wang;Xiaohong Cao;Mingguang Liu;Yunhai Liu

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The photocatalytic reduction of soluble ({text{UO}}_{2}^{2 + }) from radioactive wastewater is becoming an effective method to reduce radioactive pollution, while available catalysts are considerable limitation. Herein, the ZnS@g-C3N4 (ZSGCN) heterojunctions complexes were compounded as catalysts to reduce ({text{UO}}_{2}^{2 + }). The results from TEM, XRD, XPS, EIS, DRS and PL showed that the ZnS nanoparticles combined with graphite carbon nitride (GCN), which is the construction of heterojunctions broadened the absorption range of sunlight. The ZSGCN-5 presented the optimal photocatalytic reduction activity to ({text{UO}}_{2}^{2 + }), which was 4.34 times than that of pristine GCN. The ZSGCN-5 heterojunction becomes a promising photocatalyst for radioactive environment remediation.
The photocatalytic reduction of soluble ({text{UO}}_{2}^{2 + }) from radioactive wastewater is becoming an effective method to reduce radioactive pollution, while available catalysts are considerable limitation. Herein, the ZnS@g-C3N4 (ZSGCN) heterojunctions complexes were compounded as catalysts to reduce ({text{UO}}_{2}^{2 + }). The results from TEM, XRD, XPS, EIS, DRS and PL showed that the ZnS nanoparticles combined with graphite carbon nitride (GCN), which is the construction of heterojunctions broadened the absorption range of sunlight. The ZSGCN-5 presented the optimal photocatalytic reduction activity to ({text{UO}}_{2}^{2 + }), which was 4.34 times than that of pristine GCN. The ZSGCN-5 heterojunction becomes a promising photocatalyst for radioactive environment remediation.
DOI: 10.1039/c0ee00582g
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