Dust storms and Chinese loess sources over the last 22 million years

尘埃循环是气候的一个基本组成部分，但仍然是地球系统最不了解的方面之一。大气中的灰尘影响海洋生产力和大气二氧化碳水平、云的形成以及大气吸收或反射的辐射量，所有这些都是气候变化的驱动因素。然而，人们对过去环境变化如何控制粉尘的产生和排放知之甚少，无法量化其对气候的影响，这一事实在最近的IPCC 2007年报告中得到了承认。该项目试图通过精确定位世界上最大和最长的活跃沙尘汇--中国黄土高原的确切来源来解决这一空白。中国黄土高原包含了2200万年的黄土沉积档案，涵盖了了解地球历史的最重要时期之一。中国黄土为了解亚洲季风和沙尘暴过去的变化做出了重要贡献，是最有价值的气候档案之一。然而，它的解释依赖于这些灰尘的确切来源的详细限制，以及它到达黄土高原的路径。不幸的是，尽管使用大量样品的地球化学性质进行了调查，但在以下方面存在多种相互竞争的假设：1）准确的黄土源区，2）环境对粉尘产生的控制，3）来源是否随时间推移而变化，4）大气机制是粉尘运输，以及5）记录的最古老部分（8-22 Ma）是否确实是风吹的。这些分歧严重限制了我们对这些沉积物起源的理解，使我们无法限制过去造成尘埃排放和运输的大气、构造和海洋条件，并破坏了黄土中某些气候代用指标的使用。这反过来又限制了我们对中国过去主要环境过程的理解，以及当前大气环流系统的起源。克服这一差距的关键是适当限制黄土的来源。我们的试点工作表明，广泛应用的黄土和源区沉积物的整体沉积物地球化学分析将掩盖黄土粉尘的多个来源的细节。只有某些重矿物（比重> 2.8）的单个颗粒可以进行来源诊断，因为每个颗粒都有一个来源，并且其某些地球化学和地质年代学特征可以对此进行诊断。因此，将使用多代理单颗粒地球化学方法，以最大限度地提高成功的可能性，进行分析的多个单颗粒的锆石和其他重矿物从黄土和邻近的沙漠矿床隔离。直到我们的试点工作，这还没有进行中国黄土以前。这些分析的样品将取自中国多个典型的黄土序列，从而可以确定源随时间和空间的变化。采样将集中在关键时段，如西藏的隆升、冰河时代冰川作用的开始以及最近冰川作用强度的增强。这些结果将使我们能够测试黄土粉尘来源和运输的相互冲突的假设之间，使约束的基本控制粉尘排放和大气机制参与其传输。反过来，通过与独立记录的比较，这将使我们能够评估全球和区域气候、构造和海洋变化对尘埃的影响。目前，这是地球系统中一个知之甚少但至关重要的组成部分。最后，研究结果将测试广泛使用的沉积代用指标，如质量积累率和粒度重建过去的环境变化从黄土的有效性。

The dust cycle is a fundamental component of climate, but remains one of the least understood aspects of the Earth-system. Dust in the atmosphere affects oceanic productivity and atmospheric carbon dioxide levels, cloud formation and the amount of radiation absorbed or reflected by the atmosphere, all driving climatic change. However, how dust production and emission is controlled by environmental change in the past is poorly understood, preventing quantification of its effects on climate, fact acknowledged in the recent IPCC 2007 report. This project addresses this gap by attempting to pinpoint the precise sources of the world's largest and longest active dust sink, the Chinese Loess Plateau. The Chinese Loess Plateau contains a 22 million year archive of loess (deposited dust) deposition, covering one of the most significant time periods for understanding the Earth's history. Chinese loess has made crucial contributions to understanding past changes in the Asian monsoon and dust storms and is one of the most valuable climate archives available. However, its interpretation relies on detailed constraint of the precise sources of this dust, and the pathways by which it reaches the Loess Plateau. Unfortunately, despite investigation using the geochemical properties of bulk samples there are multiple competing hypotheses over 1) the precise loess source regions, 2) the environmental controls on dust production, 3) whether sources shift through time, 4) the atmospheric mechanisms are for dust transport and indeed 5) whether the oldest part of the record (8-22 Ma) is indeed wind-blown at all. These disagreements severely limit our understanding of the very origin of these deposits, preventing us from constraining the past atmospheric, tectonic and oceanographic conditions responsible for the emission and transport of dust and undermining the use of certain climate proxies in loess. In turn this restricts our understanding of the dominant environmental processes operating in China in the past, and the origin of the current atmospheric circulation systems. Key to overcoming this gap is to properly constrain the sources of loess. Our pilot work has demonstrated that widely applied bulk sediment geochemical analysis of sediment from loess and source regions will mask the detail of the multiple sources of loess dust. Only individual grains of certain heavy minerals (> 2.8 specific gravity) can be source diagnostic as each grain will have one source and certain of its geochemical and geochronological characteristics may be diagnostic of this. Thus analysis of multiple single grains of zircons and other heavy minerals isolated from loess and adjacent desert deposits will be undertaken using a multi-proxy single-grain geochemical approach to maximise the likelihood of success. Until our pilot work this has not been conducted on Chinese loess previously. Samples for these analyses will be taken from multiple, typical loess sequences in China, allowing determination of source variance through time and space. Sampling will concentrate on key intervals, such as the uplift of Tibet, the onset of Ice Age glaciation and the enhanced intensity of glaciation in more recent times. The results will allow us to test between conflicting hypotheses of loess dust source and transport, enabling constraint of the fundamental controls on dust emission and the atmospheric mechanisms involved in their transport. In turn and through comparison with independent records, this will allow us to assess the effect of global and regional climatic, tectonic and oceanographic changes on dust. This is currently a poorly understood yet critical component of the Earth-system. Finally, the results will test the validity of widely used sedimentary proxies such as mass accumulation rates and grain size in reconstructing past environmental changes from loess.