Electronic structure of solids and interfaces with strong electron-electron/Boson interactions

我们的研究重点是详细了解材料的化学组成，原子和电子结构及其物理特性之间的关系，包括主要由原子的价电子及其在固体中的传播决定的电，磁，光和热特性。在过渡金属和稀土化合物中，部分填充的价壳层电子具有强烈的相互作用，导致它们的自旋对齐并有序占据轨道。例如，这导致了局部磁矩和电四极矩，它们在固体中有序排列，形成有趣的磁性和轨道有序模式，具有新的和奇异的物理性质。固体中原子和离子的物理学以及电子在它们之间的传播，再加上原子的运动，是能够预测哪些结构，组合物和微观结构可以导致新的和有趣的物理性质。我们开发的理论和实验方法来详细研究这些相关电子系统的电子结构。利用加拿大光源最近开发的新的X射线光谱光束线，我们在原子尺度上研究固体的电子结构。这包括过渡金属氧化物异质结构中深埋界面的电子结构。这些接口有迷人的新特性，如超导界面之间形成的两个明智地选择父electrical insulator.We之间提出了新的方向在接口工程，利用我们新开发的分子束外延方法的新材料和接口的原子的生长。我们还建议开发一种新的世界领先的电子能量损失谱仪，具有无与伦比的能量和动量分辨率。这将与具有高能量和动量分辨率的非共振硬X射线非弹性散射互补，以确定大动量能量损失区域。这是至关重要的，以确定晶体局域场校正，这决定了电子-电子和电子声子的相互作用，在这些相关的电子系统修改的屏蔽和电子solvation effects.We还建议开发所需的理论和计算方法来解释实验结果，并预测潜在的新结构与有趣的物理性质。我们注意到，这一信息在具有非常不均匀的电子密度和极化率的系统中至关重要，就像这里感兴趣的材料中的大多数情况一样。这将在Stewart Blusson量子物质研究所的强烈合作气氛中进行，并与UBC-Max Planck-U东京量子材料中心合作。

Our research is focused on obtaining a detailed understanding of the relationship between the chemical composition, the atomic and the electronic structure of materials and their physical properties, including the electrical, magnetic, optical and thermal properties that are determined primarily by valence electrons of the atoms and their propagation in the solid. In transition metal and rare earth compounds, the partially filled valence shell electrons have strong interactions resulting in alignment of their spins and ordering the occupation of the orbitals. This leads to, for example, local magnetic moments and electrical quadrupole moments, which order in the solid to form interesting magnetic and orbital ordering patterns with new and exotic physical properties.The physics of atoms and ions in solids and the propagation of electrons between them, coupled with the motions of the atoms, lie at the heart of being able to predict which structures, compositions and micro structures could lead to new and interesting physical properties. We develop theoretical and experimental methods to study the electronic structure of these correlated electron systems in detail. With the new X-ray spectroscopy beam line recently developed at the Canadian Light Source, we study the electronic structure of solids on an atomic scale. This includes the electronic structure of deeply buried interfaces in heterostructures of transition metal oxides. These interfaces have fascinating new properties such as the superconducting interfaces formed between two judiciously selected parent electrical insulators.We propose new directions in interface engineering, utilizing our newly developed molecular beam epitaxy method for atom-by-atom growth of new materials and interfaces. We also propose the development of a new and world-leading electron energy loss spectroscopy facility with unmatched energy and momentum resolution. This will be complimented with non-resonant hard x-ray inelastic scattering with high energy and momentum resolution to determine the large momentum energy loss region. This is crucial to determine the Crystal Local Field Corrections, which determine the electron-electron and electron phonon interactions in these correlated electron systems modified by screening and electronic solvation effects.We also propose to develop the theoretical and computational methods needed to interpret the experimental result and to predict potentially new structures with interesting physical properties. We note that this information is of crucial importance in systems that have a very non-uniform electron density and polarizability, as is mostly the case in the materials of interest here. This will be done in the strongly collaborative atmosphere of the Stewart Blusson Quantum Matter Institute and in collaboration with the UBC-Max Planck-U Tokyo Centre for Quantum Materials.