In situ synchrotron X-ray diffraction study on epitaxial-growth dynamics of III–V semiconductors

In situ synchrotron X-ray diffraction study on epitaxial-growth dynamics of III–V semiconductors
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III-V族半导体外延生长动力学的原位同步加速器X射线衍射研究

DOI:
10.7567/jjap.57.050101
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发表时间:
2018
影响因子:
1.5
通讯作者:
M. Takahasi
M. Takahasi
中科院分区:
物理与天体物理4区
文献类型:
--
作者:
M. Takahasi

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结合衍射理论和仪器背景,对原位同步辐射X射线衍射(XRD)在Ⅲ-Ⅴ族半导体分子束外延(MBE)生长中的应用进行了沿着综述。X射线不仅对生长膜的表面敏感,而且对掩埋的界面结构也敏感,因为它们的穿透深度很大。此外,高达微米量级的空间相干长度使X射线广泛适用于表征低维结构,如量子点和线。在生长过程中的原位XRD研究进行了使用X射线衍射仪,这是与MBE室相结合。X射线倒易空间映射的速度匹配一个典型的增长率,实现了使用强烈的X射线可从同步加速器光源和区域检测器。的重要性,测量的三维分布的XRD强度在倒易空间图的MBE生长的两个,一个,和零维结构证明。三维X射线倒易映射提供了大量关于二维InGaAs/GaAs(001)外延薄膜生长过程的信息,包括各向异性应变弛豫、组分不均匀性以及表面和界面粗糙度的演变。对于一维GaAs纳米线生长在Au催化的气-液-固模式,纳米线的直径和多型体的形成之间的关系已建议在原位XRD测量的基础上。原位三维X射线倒易空间映射也被证明是有用的,用于确定的横向和纵向尺寸的自组装InAs/GaAs(001)量子点,以及在生长过程中的内部应变分布。
The application of in situ synchrotron X-ray diffraction (XRD) to the molecular-beam epitaxial (MBE) growth of III–V semiconductors is overviewed along with backgrounds of the diffraction theory and instrumentation. X-rays are sensitive not only to the surface of growing films but also to buried interfacial structures because of their large penetration depth. Moreover, a spatial coherence length up to µm order makes X-rays widely applicable to the characterization of low-dimensional structures, such as quantum dots and wires. In situ XRD studies during growth were performed using an X-ray diffractometer, which was combined with an MBE chamber. X-ray reciprocal space mapping at a speed matching a typical growth rate was achieved using intense X-rays available from a synchrotron light source and an area detector. The importance of measuring the three-dimensional distribution of XRD intensity in a reciprocal space map is demonstrated for the MBE growth of two-, one-, and zero-dimensional structures. A large amount of information about the growth process of two-dimensional InGaAs/GaAs(001) epitaxial films has been provided by three-dimensional X-ray reciprocal mappings, including the anisotropic strain relaxation, the compositional inhomogeneity, and the evolution of surface and interfacial roughness. For one-dimensional GaAs nanowires grown in a Au-catalyzed vapor-liquid–solid mode, the relationship between the diameter of the nanowires and the formation of polytypes has been suggested on the basis of in situ XRD measurements. In situ three-dimensional X-ray reciprocal space mapping is also shown to be useful for determining the lateral and vertical sizes of self-assembled InAs/GaAs(001) quantum dots as well as their internal strain distributions during growth.
DOI: 10.1002/pssc.201000508
发表时间: 2011
期刊: Physica Status Solidi(c)
影响因子: --
作者:
H. Tameoka;T. Kawase;M. Tabuchi;and Y. Takeda
通讯作者: and Y. Takeda
DOI: 10.1063/1.110199
发表时间: 1993-12-06
影响因子: 4
作者:
LEONARD, D;KRISHNAMURTHY, M;PETROFF, PM
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DOI: 10.1021/acs.cgd.5b00915
发表时间: 2015-09
影响因子: 3.8
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M. Takahasi;M. Kozu;T. Sasaki;Wen Hu
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In As/GaAs(001)量子点分子束外延生长的原位X射线衍射研究
DOI: --
发表时间: --
影响因子: 1.8
作者:
M.Takahasi;J.Mizuki
通讯作者: J.Mizuki
DOI: 10.1038/nature17148
发表时间: 2016-03-17
期刊: Nature
影响因子: 64.8
作者:
Jacobsson D;Panciera F;Tersoff J;Reuter MC;Lehmann S;Hofmann S;Dick KA;Ross FM
通讯作者: Ross FM