Thickness effects of Bi0.89Ti0.11FeO3 thin films deposited on PbZr0.2Ti0.79Nb0.01O3 buffer layers

Thickness effects of Bi0.89Ti0.11FeO3 thin films deposited on PbZr0.2Ti0.79Nb0.01O3 buffer layers
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PbZr0.2Ti0.79Nb0.01O3 缓冲层上沉积 Bi0.89Ti0.11FeO3 薄膜的厚度效应

DOI:
10.1016/j.jallcom.2010.09.049
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发表时间:
2011-01
影响因子:
6.2
通讯作者:
W.B. Wu
W.B. Wu
中科院分区:
材料科学2区
文献类型:
--
作者:
X.M. Chen;G.D. Hu;J.C. Wang;L. Cheng;C.H. Yang;W.B. Wu

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采用金属有机物分解法在40 nm厚的PbZr0.2Ti0.79Nb0.01O3(PZTN)缓冲Pt(111)/Ti/SiO2/Si衬底上制备了厚度为200- 440 nm的Bi0.89Ti0.11FeO3薄膜。由于PZTN缓冲层具有良好的绝缘性能和高的击穿特性,Bi_(0.89)Tb_(0.11)FeO_3薄膜的漏电流显著降低。所有薄膜均表现出良好的饱和和矩形的P-E磁滞回线,没有任何明显的泄漏行为。所有Bi_(0.89)Ti_(0.11)FeO_3薄膜的剩余极化强度Pr和矫顽场E_c分别为45-50μC/cm ~ 2和200 kV/cm,且对薄膜厚度的依赖性很弱。200 nm厚的Bi 0.89 Ti 0.11 FeO 3薄膜具有较好的抗疲劳特性和电荷保持能力,PZTN缓冲层的抗老化能力较强,显著抑制了畴反转。
Bi0.89Ti0.11FeO3thin films with the thicknesses of 200–440nm were fabricated on the 40-nm-thick PbZr0.2Ti0.79Nb0.01O3(PZTN)-buffered Pt(111)/Ti/SiO2/Si substrates using a metal organic decomposition process. As a result of the good insulating property and high breakdown characteristic of the PZTN buffer layer, the leakage currents in the Bi0.89Tb0.11FeO3films are significantly reduced. All the films show well-saturated and rectangular P–E hysteresis loops without any evident leaky behavior. The remnant polarization Prand coercive field Ecfor all Bi0.89Ti0.11FeO3films are around 45–50μC/cm2and 200kV/cm, respectively, and show weak dependent on the film thickness. The 200-nm-thick Bi0.89Ti0.11FeO3film exhibits better fatigue-free characteristic and charge-retaining ability, and the domain backswitching is significantly restrained due to the strong anti-aging ability of the PZTN buffer layer.
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