Laser Spectroscopy Probing of Excitation and Coherence Dynamics

为了继续他们在激光光谱探测方面的努力， 激发和相干过程，他们建议使用这个 续发补助金，以进行以下领域的研究： 电子和激发转移的超短时间动力学 凝聚介质中的模型系统;（B）选择性脉冲激发 研究连贯性和松弛过程;以及 (c)微观溶剂化的激光光谱学研究 聚类 他们将在这项研究中使用的技术 （已经在他们的实验室中使用）是皮秒， 飞秒光谱学，多脉冲光激发，激光 方法和多光子（TOF和PES）检测方法。 他们的 目标是应用（和修改）这些技术来学习 关于能量弛豫、溶剂化和相干的动力学 在压缩介质中，并检查皮秒和飞秒 经历（微观）溶剂化的分子动力学， 集群形成

In continuation of their efforts on laser spectroscopy probing of excitation and coherence processes, they propose to use this renewal grant to undertake research in the following areas: (a) ultrashort time dynamics of electron and excitation transfer in model systems in condensed media; (b) selective-pulse excitation for the invesitgation of coherence and relaxation processes; and (c) laser spectroscopy studies of microscopic solvation and clustering. The techniques that they shall use in this research (which are already used in their laboratory) are picosecond and femtosecond spectroscopy, multiple pulse optical excitation methods, and multiphoton (TOF and PES) detection methods. Their objectives are to apply (and modify) these techniques to learn about the dynamics of energy relaxation, solvation, and coherence in condensed media, and to examine the picosecond and femtosecond dynamics of molecules undergoing (microscopic) solvation and clustering formation.