Collaborative Research: Analyses, Measurements and Modeling in Support of the Asian Monsoon Chemical and Climate Impact Project (ACCLIP)

合作研究：支持亚洲季风化学和气候影响项目 (ACCLIP) 的分析、测量和建模

• 批准号: 1853929
• 负责人: Laura Pan
• 金额: $ 59.68万
• 依托单位: University Corporation For Atmospheric Res
• 依托单位国家: 美国
• 项目类别: Standard Grant
• 财政年份: 2019
• 资助国家: 美国
• 起止时间: 2019-05-15 至 2024-10-31
• 项目状态: 已结题
• 来源: https://www.nsf.gov/awardsearch/showAward?AWD_ID=1853929&HistoricalAwards=false
• 关键词: Collaborative; Research; Analyses; Measurements; Modeling

This effort involves an aircraft study of the chemistry and dynamics of the Asian Summer Monsoon (ASM). This atmospheric circulation takes place in the upper troposphere and lower stratosphere and spans the Pacific Ocean east of Asia westward to the Middle East. The vertical transport of pollutants within the ASM can have a global impact on atmospheric chemistry and radiation. This project includes the training of graduate students and post-doctoral scientists.The four main objectives of the project are: (1) Investigate the transport pathway of the ASM uplifted air from inside of the anticyclone to the global upper troposphere-lower stratosphere (UTLS); (2) Sample the chemical content of air processed in the ASM to ascertain its role in UTLS ozone chemistry, and in re-distributing active species and short-lived climate forcers to examine the respective roles of Asian pollution and the monsoon strength in chemistry and climate, and to understand two-way coupling between chemistry and climate. Chemical tracers of different lifetimes can also help characterize the ASM uplifting time scales, which are difficult for the models to estimate; (3) Obtain information on aerosol size, mass and chemical composition necessary for determining the radiative impact of the ASM, for constraining models of aerosol formation and for contrasting the organic-rich ASM UTLS aerosol population with that of sulfate-rich volcanic plumes and the background aerosol population; and (4) Measure the water vapor distribution associated with the monsoon dynamical structure to evaluate transport across the tropopause, and determine the role of the ASM in water vapor transport into the stratosphere.This project is scheduled to take place during July-August 2020 and will establish and expand collaborations between several academic institutions, government partners, and international institutions.This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.

这项工作涉及对亚洲夏季风(ASM)的化学和动力学进行飞机研究。这种大气环流发生在对流层上层和平流层下层，并横跨太平洋，从亚洲以东向西一直到中东。ASM内污染物的垂直输送可对大气化学和辐射产生全球影响。该项目包括对研究生和博士后科学家的培训。项目的四个主要目标是：(1)调查ASM上升的空气从反气旋内部到全球对流层上部平流层下部(UTLS)的输送路径；(2)采样ASM中处理的空气的化学成分，以确定其在UTLS臭氧化学中的作用，并重新分配活性物种和短暂的气候作用力，以研究亚洲污染和季风强度在化学和气候中的各自作用，并了解化学和气候之间的双向耦合。不同寿命的化学示踪剂也有助于表征ASM抬升的时间尺度，模式难以估计；(3)获得有关气溶胶大小、质量和化学成分的信息，以确定ASM的辐射影响，约束气溶胶形成模式，并将富有机的ASM UTLS气溶胶种群与富硫酸盐火山羽流和背景气溶胶种群进行对比；和(4)测量与季风动力结构有关的水汽分布，以评估穿过对流层顶的输送，并确定ASM在水汽输送到平流层中的作用。该项目计划于2020年7-8月进行，将建立和扩大几个学术机构、政府合作伙伴和国际机构之间的合作。该奖项反映了NSF的法定使命，并通过使用基金会的智力价值和更广泛的影响审查标准进行评估，被认为值得支持。

项目成果

Diagnostics of Convective Transport Over the Tropical Western Pacific From Trajectory Analyses

• DOI: 10.1029/2020jd034341
• 发表时间: 2021-09
• 期刊: Journal of Geophysical Research
• 作者: Warren P. Smith;L. Pan;S. Honomichl;S. Chelpon;R. Ueyama;L. Pfister

East Asian summer monsoon delivers large abundances of very short-lived organic chlorine substances to the lower stratosphere

• DOI: 10.1073/pnas.2318716121
• 发表时间: 2024-03-19
• 期刊: PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
• 影响因子: 11.1
• 作者: Pan，Laura L.;Atlas，Elliot L.;Newman，Paul A.
• 通讯作者: Newman，Paul A.

Evaluating the Model Representation of Asian Summer Monsoon Upper Troposphere and Lower Stratosphere Transport and Composition Using Airborne In Situ Observations

• DOI: 10.1029/2023jd039756
• 发表时间: 2024-02-28
• 期刊: JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
• 影响因子: 4.4
• 作者: Smith，Warren P.;Pan，Laura L.;Ravegnani，Fabrizio
• 通讯作者: Ravegnani，Fabrizio

A Multimodel Investigation of Asian Summer Monsoon UTLS Transport Over the Western Pacific

• DOI: 10.1029/2022jd037511
• 发表时间: 2022-12
• 期刊: Journal of Geophysical Research: Atmospheres
• 作者: L. Pan;D. Kinnison;Q. Liang;M. Chin;M. Santee;J. Flemming;Warren P. Smith;S. Honomichl;J. Bresch;L. Lait;Yunqian Zhu;S. Tilmes;P. Colarco;J. Warner;Adrien Vuvan;C. Clerbaux;E. Atlas;P. Newman;T. Thornberry;W. Randel;O. B. Toon