Towards a Unified Framework of Quantum Dynamics of Nonlinear Optical and Transport Processes

建立非线性光学和传输过程量子动力学的统一框架

• 批准号: 2015639
• 负责人: Benjamin M. Fregoso
• 金额: $ 40万
• 依托单位: Kent State University
• 依托单位国家: 美国
• 项目类别: Continuing Grant
• 财政年份: 2021
• 资助国家: 美国
• 起止时间: 2021-01-01 至 2024-12-31
• 项目状态: 已结题
• 来源: https://www.nsf.gov/awardsearch/showAward?AWD_ID=2015639&HistoricalAwards=false
• 关键词: Towards; Unified; Framework; Quantum; Dynamics

Nontechnical summaryThis project advances and broadens our basic scientific understanding of materials under intense illumination. Of interest are phenomena and materials where the laws of physics are radically distinct from day-to-day experience due to the smallness of particles inside materials, i.e., quantum physics and quantum materials. Advancing our knowledge of irradiated quantum materials will facilitate their use in future quantum technologies, e.g., more efficient solar energy harvesting, faster computers and optoelectronic applications. This research develops new concepts and methods in both optics and quantum condensed matter physics, benefiting both fields of knowledge. Education and outreach efforts include developing a new computational physics course, hosting a workshop for senior undergraduate students (including those from nearby minority-serving institutions), developing a one-day STEM curriculum unit for low-income high school students enrolled in Upward Bound, hosting middle school teachers via the US State Department’s International Leaders in Education Program, and mentoring undergraduates and graduate students in research. These efforts aim to expand and diversify the STEM workforce.Technical summaryThe need for clean energy sources has led to great interest in solar energy harvesting. Unconventional photovoltaic mechanisms such as the so-called bulk photovoltaic effect are promising candidates for both solar energy harvesting and novel optoelectronic applications. Key aspects of the bulk photovoltaic effect, however, are not well understood. This project aims to develop a theoretical framework to classify and unify nonlinear transport in crystalline solids including the bulk photovoltaic effect. Materials of interest include two-dimensional ferroelectrics and topological materials. The framework will ascertain the role of dissipation and carrier interactions not yet addressed in existing analytical or numerical theories but which are important to understand experiments and uncover novel nonlinear phenomena. The project uses analytical field theoretic methods and numerical density functional approaches.In a related topic, light is also emerging as a versatile tool for engineering the properties of materials as exemplified by the recent realization of the Floquet-Bloch state and the light-induced anomalous Hall effect. These states are very short-lived because irradiated materials quickly heat up. Understanding pathways to thermalization is of fundamental importance in realizing applications of novel nonequilibrium states. The PI will construct models of many-body thermalization which include electron interactions, excitons and phonons and in so doing assess the opportunities and challenges of laser-driven nonequilibrium states in realistic scenarios. Theoretical models will be experimentally validated via close collaboration with partners conducting experimental research.This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.

非技术性总结这个项目推进和拓宽了我们对强光下材料的基本科学理解。 感兴趣的是物理定律与日常经验截然不同的现象和材料，这是由于材料内部的粒子很小，即，量子物理和量子材料。提高我们对辐照量子材料的认识将促进它们在未来量子技术中的应用，例如，更高效的太阳能收集，更快的计算机和光电应用。这项研究开发了光学和量子凝聚态物理学的新概念和方法，使这两个知识领域受益。教育和推广工作包括开发一门新的计算物理课程，为高年级本科生举办研讨会，（包括来自附近少数民族服务机构的学生），为参加“向上成长”的低收入高中生开发一个为期一天的STEM课程单元，通过美国国务院的国际教育领袖计划接待中学教师，并指导本科生和研究生进行研究。这些努力旨在扩大STEM劳动力并使其多样化。技术概述对清洁能源的需求导致人们对太阳能收集产生了极大的兴趣。非传统的光伏机制，如所谓的体光伏效应是有前途的候选人的太阳能收集和新型光电应用。然而，体光伏效应的关键方面还没有得到很好的理解。本计画旨在发展一个理论架构来分类和统一结晶固体中的非线性输运，包括体光生伏打效应。感兴趣的材料包括二维铁电体和拓扑材料。该框架将确定耗散和载流子相互作用的作用尚未解决现有的分析或数值理论，但这是重要的理解实验和发现新的非线性现象。该项目使用分析场论方法和数值密度泛函方法。在相关主题中，光也正在成为工程材料特性的多功能工具，例如最近实现的Floquet-Bloch态和光诱导反常霍尔效应。这些状态是非常短暂的，因为辐射材料迅速升温。理解热化的途径对于实现新的非平衡态的应用具有根本的重要性。PI将构建多体热化模型，其中包括电子相互作用，激子和声子，并在这样做时评估现实场景中激光驱动非平衡态的机会和挑战。该奖项反映了NSF的法定使命，并通过使用基金会的知识价值和更广泛的影响审查标准进行评估，被认为值得支持。

项目成果

Ultrafast relaxation of acoustic and optical phonons in a topological nodal-line semimetal ZrSiS

• DOI: 10.1038/s42005-022-00980-6
• 发表时间: 2021-11
• 期刊: Communications Physics
• 影响因子: 5.5
• 作者: Yangyang Liu;Gyanendra Dhakal;Anup Pradhan Sakhya;John E. Beetar;Firoz Kabir;Sabin Regmi;D. Kaczorowski;M. Chini;Benjamin M. Fregoso;M. Neupane

Pure spin current injection of single-layer monochalcogenides

单层单硫属化物的纯自旋电流注入

• DOI: 10.1088/2053-1591/acbf99
• 发表时间: 2023
• 期刊: Materials Research Express
• 影响因子: 2.3
• 作者: Mendoza, Bernardo S;Grillo, Simone;Juárez-Reyes, Lucila;Fregoso, Benjamin M
• 通讯作者: Fregoso, Benjamin M

Energy relaxation dynamics in a nodal-line semimetal

节线半金属中的能量弛豫动力学

• DOI: 10.1103/physrevb.105.144304
• 发表时间: 2022
• 期刊: Physical Review B
• 影响因子: 3.7
• 作者: Fregoso, Benjamin M.;Neupane, Madhab;Sakhya, Anup Pradhan
• 通讯作者: Sakhya, Anup Pradhan

Bulk photospin effect: Calculation of electric spin susceptibility to second order in an electric field

• DOI: 10.1103/physrevb.106.195108
• 发表时间: 2022-03
• 期刊: Physical Review B
• 影响因子: 3.7
• 作者: Benjamin M. Fregoso