Controlling Exchange and Quenched Disorder in Low-Dimensional Spin Systems

研究新材料的结构和物理特性是开发创新产品和技术的基础，因此对社会非常重要，因为这些知识产生附加值。我们快速发展的经济需要对新材料的物理特性进行更系统的分析，以便在修改其成分时对其进行正确的理解。这允许通过专门使用这些新发现来开发新产品来增强技术优势。因此，研究不应仅仅强调新材料的开发，而应了解如何开发具有预定特征的特定材料。通过合成和表征组成和关系，阐明确定相关总系统的集体行为的有序机制，获得对物理性质修改方案的见解。此外，由于量子临界点周围的相模型可以通过非热控制参数实现，淬火无序可以导致具有有趣的新特性的奇异临界点。本研究计划“控制低维自旋系统中的交换与淬灭无序”，主要研究中子散射的相关性。本文研究了由歌德大学的研究员设计和生长的三个低维自旋系统，它们非常适合于本研究项目：a）在模型各向异性的三角晶格材料Cs_2CuCl_（4-x）Br_x上，我们研究了准一维阻挫系统中的猝灭无序效应; B）在新的金属-有机化合物K（C_8H_（16）O_4）_2CuCl_3 H_2 O上，我们将研究相互作用的量子二聚体单元中的自旋相关，c）在Ba_（1-x）Sr_xCuSi_2 O_6中，我们将探索在二维量子临界点的玻色-爱因斯坦凝聚的令人兴奋的物理。

Investigation of structural and physical properties of new materials is the basis for the development of innovative products and technologies and therefore of high importance for the society as this knowledge produces an added value. Our rapidly evolving economy requires an even more systematic analysis of the physical properties of new materials to gain a sound understanding thereof in case of a modification of their composition. This allows enhancing technological ascendancy by specifically using such new findings for the development of new products. Therefore, research should not emphasis merely on the development of new materials, but on the understanding how to develop specific materials with pre-defined characteristics. Insights into the scheme of modification of physical properties are gained through synthesis and characterization of compositions and relations, elucidating the ordering mechanism, which determines the collective behavior of i.e. a correlated total system. Furthermore, as modeling of phases around quantum critical points are realizable through nonthermal control parameter, quenched disorder can lead to exotic critical points with interesting new properties. This research project Controlling Exchange and Quenched Disorder in Low-Dimensional Spin Systems focuses on the investigation of correlations by neutron scattering. It deals with the following three low-dimensional spin systems, designed and grown by the fellow at Goethe-University and which are very well suited for this research project: a) on the model-anisotropic triangular lattice material Cs2CuCl4-xBrx we study the effects of quenched disorder in quasi-one-dimensional frustrated systems; b) on the new metal-organic compound K(C8H16O4)2CuCl3 H2O we will investigate spin-correlations in interacting quantum dimer units, and c) in Ba1-xSrxCuSi2O6 we will explore the exciting physics of Bose-Einstein condensation at a two-dimensional quantum critical point.