Development of Cavity-Dumped Ti : sapphire Femtosecond Laser and its Amplifier
Development of Cavity-Dumped Ti : sapphire Femtosecond Laser and its Amplifier
批准号:
10554034
负责人:
TOMINAGA Keisuke
金额:
$8.7万
依托单位:
依托单位国家:
日本
项目类别:
Grant-in-Aid for Scientific Research (B)
财政年份:
1998
资助国家:
日本
项目状态:
已结题
起止时间:
1998 至 1999
中文摘要
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英文摘要
We have developed an intra-cavity dumped femtosecond Ti : sapphire laser system and its multi-pass amplifier to obtain a moderately high energy short pulse, enough to perform third order optical nonlinear experiment in liquid solutions. Currently, commercially available femtosecond Ti : sapphire laser systems are either (1)Ti : sapphire oscillator (general price = 18,000,000 yen), which yields a pulse with an energy of 4 nJ/pulse, or (2)Ti : sapphire oscillator and its amplifier (general price = 50,000,000 yen), which yields a pulse with an energy of 1 mJ/pulse. In order to perform experiment with a short pulse in chemical systems such as transient absorption or photon echo, we need a pulse with an energy around mJ/pulse to sub mJ/pulse. Therefore, a new short pulse laser system is desirable to get s moderately high energy pulse. In this research project we here calculated stability of oscillation for the cavity-dumped Ti : sapphire laser by the ABCD matrix formalism. We have investigated both the five-mirror configuration and six-mirror configuration theoretically and experimentally. The cavity dumper laser produces a pulse width of 13 fs and energy of 67 nJ/pulse at 4 MHz. Currently, a multi-pass (six-pass) amplifier with a Ti : sapphire crystal is being designed and constructed to get a higher energy pulse. The purpose of this amplifier is to get a pulse with an energy more than sub microJ/pulse at 20 kHz. We are also writing a manual to construct this laser system and are planning to distribute it to public.
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K.Ohta, T.J.Kang, K.Tominaga, and K.Yoshihara: "Femtosecond Time-resolved Fluorescence Studies of a Dye Molecule in Solution : Ultrafast Processes from a Higher Excited Electronic State"Chem. Phys.. 242. 103-114 (1999)
K.Ohta、T.J.Kang、K.Tominaga 和 K.Yoshihara:“溶液中染料分子的飞秒时间分辨荧光研究:来自更高激发电子态的超快过程”Chem。
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K.Tominaga and H.Maekawa: "Development of Two-Dimensional Raman Spectroscopy by Higher-Order Optical Nonlinear Spectroscopy"J. Luminescence. (in press.).
K.Tominaga 和 H.Maekawa:“通过高阶光学非线性光谱开发二维拉曼光谱”J。
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H. Shirota: ""Substituent Effect and Deuterium Isotope Effect of Ultrafast Intermolecular Electron Transfer : Coumarin in Electron Donating Solvent""J. Phys. Chem. A. 102. 3089-3102 (1998)
H. Shirota:“超快分子间电子转移的取代基效应和氘同位素效应:给电子溶剂中的香豆素”J。
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K.Tominaga: "Recent Development of Nonlinear Spectroscopy in Liquids"Laser Chem.. 19. 117-122 (1999)
K.Tominaga:“液体中非线性光谱学的最新发展”Laser Chem.. 19. 117-122 (1999)
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K.Tominaga: "Development of two-Dimensional al Raman Spectroscopy by Higher-Order Optical Nonlinear Spectroscopy"Journal of Lumimescience. (in press).
K.Tominaga:“通过高阶光学非线性光谱开发二维拉曼光谱”Lumimescience 杂志。
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