Syntheses and function controls of single-molecule-based photo-hydrogen-evolving molecular devices

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Studies on visible light induced water-splitting reactions are important in order to achieve the systems to convert solar energy into hydrogen energy. In this study, we tackled syntheses and functional controls of single-molecule-based photo-hydrogen-evolving molecular devices, which have both photosensitizing and H2-evolving abilities. In the result, we could succeed in unveiling the factors controlling the activities of molecular devices. We also succeeded in developing the bifunctional platinum complexes promoting photochemical H2 production from water in one component.