Atmospheric Chemistry In The Earth System (ACITES) Network

地球系统大气化学 (ACITES) 网络

• 批准号: NE/K001329/1
• 负责人: David Stevenson
• 金额: $ 20.83万
• 依托单位: University of Edinburgh
• 依托单位国家: 英国
• 项目类别: Research Grant
• 财政年份: 2013
• 资助国家: 英国
• 起止时间: 2013 至 无数据
• 项目状态: 已结题
• 来源: https://gtr.ukri.org/projects?ref=NE%2FK001329%2F1
• 关键词: Atmospheric; Chemistry; Earth; System; ACITES

Atmospheric chemistry plays an essential role in the Earth system. Whether from the perspective of a changing radiation balance, the impact of pollutants on vegetation, the size distribution of cloud droplets or the effect of desert dust on ocean bio-geochemistry, understanding the composition and chemistry of the atmosphere is vital. The UK has a long history in atmospheric chemistry research, from the early days of sulphur smogs, through stratospheric ozone depletion to ongoing research on air quality and climate. The UK community is diverse and plays a central role in global efforts to advance understanding through laboratory, field and process modelling studies.Much of this world-leading atmospheric chemistry research focuses on developing detailed understanding of the various processes controlling atmospheric composition. However, addressing many of society's greatest environmental problems now requires a wider 'Earth System' approach which considers the ensemble of processes occurring on the planet, from the biosphere, to the oceans, cryosphere and the atmosphere, rather than focusing on a single domain in isolation. Earth System Models represent our understanding of processes and interactions across these domains and creating such models is one of the grand challenges for science. Achieving an effective integration of state-of-the-science understanding derived from process studies into Earth System Models is a challenge. This network will encourage this integration in order to better develop the UK's capabilities in atmospheric chemistry and Earth System Modelling. The network will achieve this exchange in two main ways. The first will be through a series of meetings, the second will be through the community undertaking two science projects. The first activity will be a comprehensive series of meetings bring together the various processes focused groups with Earth System Modelling focused groups. These will include groups from universities, NERC Centres and Meteorological Services. These will include both large, multi-day inclusive meetings to bring together the whole community and smaller, more focused meetings. The three large meetings will discuss science topics and future directions. They will identify important science topics which will be followed up with smaller focused meetings (~12). Although the topics of the majority of these meetings will be chosen at the large meetings, three have been chosen in advance. One of these involves reactive carbon emissions from the biosphere and two involve the atmospheric chemistry schemes used within models of different complexities. The network will also undertake two challenging science projects supported by two PDRA posts. These focus on developing observationally constrained metrics of two key processes for atmospheric chemistry: transport and deposition. Both of these processes need to be 'fit for purpose' for ESMs to be suitable for atmospheric chemistry studies. Groups across the country, including those running ESMs, will provide relevant model simulations. Observationally based metrics will be constructed and the models compared to assess their suitability. Other activities will include workshops to allow process focused scientists to engage with the current generation of NERC/MO ESM; meetings to discuss technical/software/governance issues with ESMs; support for the network to engage with similar international efforts; and the creation of an Emerging Scientists network to foster the next generation of scientists.

大气化学在地球系统中起着至关重要的作用。无论是从辐射平衡的变化、污染物对植被的影响、云滴的大小分布还是沙漠尘埃对海洋生物地球化学的影响的角度来看，了解大气的组成和化学性质都至关重要。英国在大气化学研究方面有着悠久的历史，从早期的硫磺烟雾，到平流层臭氧消耗，再到正在进行的空气质量和气候研究。英国社区是多元化的，并在全球努力通过实验室，现场和过程建模研究促进理解中发挥着核心作用。许多世界领先的大气化学研究侧重于发展控制大气成分的各种过程的详细了解。然而，解决许多社会上最大的环境问题，现在需要一个更广泛的“地球系统”的方法，考虑整体的过程发生在地球上，从生物圈，海洋，冰冻圈和大气层，而不是集中在一个孤立的域。地球系统模型代表了我们对这些领域的过程和相互作用的理解，创建这样的模型是科学的重大挑战之一。将过程研究得出的最新科学认识有效地整合到地球系统模型中是一项挑战。该网络将鼓励这种整合，以便更好地发展联合王国在大气化学和地球系统建模方面的能力。该网络将通过两种主要方式实现这种交换。第一个将通过一系列会议，第二个将通过社区承担两个科学项目。第一项活动将是一系列综合会议，将各进程重点小组与地球系统建模重点小组聚集在一起。这些将包括来自大学、NERC中心和气象服务的团体。这些会议将包括将整个社区聚集在一起的大型、为期多天的包容性会议，以及更有重点的小型会议。这三个大型会议将讨论科学主题和未来方向。他们将确定重要的科学主题，这些主题将通过较小的重点会议（~12）跟进。虽然大多数会议的议题将在大型会议上选定，但有三个议题是事先选定的。其中一个涉及生物圈的活性碳排放，两个涉及不同复杂性模型中使用的大气化学方案。该网络还将开展两个具有挑战性的科学项目，由两个PDRA职位提供支持。这些项目侧重于制定大气化学两个关键过程的观测约束指标：传输和沉积。这两个过程都需要“适合于目的”，使ESM适合于大气化学研究。全国各地的团体，包括那些运行ESM的团体，将提供相关的模型模拟。将构建基于观测的指标，并对模型进行比较，以评估其适用性。其他活动将包括：举办讲习班，让注重进程的科学家参与当前一代的NERC/MO无害环境管理;举行会议，与无害环境管理机制讨论技术/软件/治理问题;支持网络参与类似的国际努力;以及创建一个新兴科学家网络，以培养下一代科学家。

项目成果

Evaluation of ACCMIP outgoing longwave radiation from tropospheric ozone using TES satellite observations

• DOI: 10.5194/acp-13-4057-2013
• 发表时间: 2013-04
• 期刊: Atmospheric Chemistry and Physics
• 影响因子: 6.3
• 作者: K. W. Bowman;D. Shindell;H. Worden;J. Lamarque;Paul Young;David Stevenson;Z. Qu;M. D. L. Torre;D. Bergmann;P. Cameron-smith;William J. Collins;R. M. Doherty;S. Dalsøren;G. Faluvegi;G. Folberth;L. Horowitz;B. Josse;Y. Lee;Ian A. MacKenzie;G. Myhre;Tatsuya Nagashima;V. Naik;David A Plummer;S. Rumbold;R. Skeie;S. Strode;K. Sudo;S. Szopa;A. Voulgarakis;G. Zeng;S. Kulawik;A. Aghedo;John R. Worden

Effects of global change during the 21st century on the nitrogen cycle

• DOI: 10.5194/acp-15-13849-2015
• 发表时间: 2015-01-01
• 期刊: ATMOSPHERIC CHEMISTRY AND PHYSICS
• 影响因子: 6.3
• 作者: Fowler, D.;Steadman, C. E.;Galloway, J. N.
• 通讯作者: Galloway, J. N.

Multi-model mean nitrogen and sulfur deposition from the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP): evaluation of historical and projected future changes

• DOI: 10.5194/acp-13-7997-2013
• 发表时间: 2013-01-01
• 期刊: ATMOSPHERIC CHEMISTRY AND PHYSICS
• 影响因子: 6.3
• 作者: Lamarque, J-F;Dentener, F.;Nolan, M.
• 通讯作者: Nolan, M.

Peroxy acetyl nitrate (PAN) measurements at northern midlatitude mountain sites in April: a constraint on continental source-receptor relationships

4月份北部中纬度山区的过氧乙酰硝酸盐（PAN）测量：对大陆源-受体关系的限制

• DOI: 10.5194/acp-18-15345-2018
• 发表时间: 2018
• 期刊: Atmospheric Chemistry and Physics
• 影响因子: 6.3
• 作者: Fiore A

Is the ozone climate penalty robust in Europe?

• DOI: 10.1088/1748-9326/10/8/084015
• 发表时间: 2015-08-01
• 期刊: ENVIRONMENTAL RESEARCH LETTERS
• 影响因子: 6.7
• 作者: Colette, Augustin;Andersson, Camilla;Young, Paul
• 通讯作者: Young, Paul