Bioelectronic interfaces by spontaneously organized peptides on 2D atomic single layer materials.
Bioelectronic interfaces by spontaneously organized peptides on 2D atomic single layer materials.
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DOI:
10.1038/srep33778
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发表时间:
2016-09-22
影响因子:
4.6
通讯作者:
Sarikaya M
中科院分区:
文献类型:
--
作者:
Hayamizu Y;So CR;Dag S;Page TS;Starkebaum D;Sarikaya M
Self-assembly of biological molecules on solid materials is central to the “bottom-up” approach to directly integrate biology with electronics. Inspired by biology, exquisite biomolecular nanoarchitectures have been formed on solid surfaces. We demonstrate that a combinatorially-selected dodecapeptide and its variants self-assemble into peptide nanowires on two-dimensional nanosheets, single-layer graphene and MoS2. The abrupt boundaries of nanowires create electronic junctions via spatial biomolecular doping of graphene and manifest themselves as a self-assembled electronic network. Furthermore, designed peptides form nanowires on single-layer MoS2 modifying both its electric conductivity and photoluminescence. The biomolecular doping of nanosheets defined by peptide nanostructures may represent the crucial first step in integrating biology with nano-electronics towards realizing fully self-assembled bionanoelectronic devices.
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