Coherent spectroscopic investigations of dynamic hydrogen bond structures in hydrated clusters

这项研究的最终目的是实时观察氢键动力学，如伸缩、解离和重排。我成功地利用所谓的信使调节冷却技术调节了水合团簇的分子间振动动力学。此外，为了实时观察分子动力学，我利用我的独特概念设计了一台飞秒时间分辨离子/电子成像装置。我希望这些成果能促进对分子动力学的进一步研究。

The ultimate purpose of this study was real-time observations of hydrogen bond dynamics such as stretchings, dissociations, and rearrangements. I succeeded in tuning intermolecular vibration dynamics of hydrated clusters using so-called messenger-mediated cooling technique. In addition, for real-time observation of molecular dynamics, I designed a femtosecond time-resolved ion/electron imaging setup utilizing my unique concept. I hope these achievements stimulate further studies of molecular dynamics.