Quantum teleportation of radical pair in photosynthetic biomembrane
Quantum teleportation of radical pair in photosynthetic biomembrane
批准号:
22654051
负责人:
MINO Hiroyuki
金额:
$2.05万
依托单位:
依托单位国家:
日本
项目类别:
Grant-in-Aid for Challenging Exploratory Research
财政年份:
2010
资助国家:
日本
项目状态:
已结题
起止时间:
2010 至 2012
中文摘要
为了研究生物膜之间的量子隐形传输,我们对光系统II中的自由基对进行了测试。为了实现这一目的,在8.5-10.5 GHz范围内,多个微波频率被用于脉冲电子顺磁共振(EPR)的自旋激发。将五种不同的微波频率馈入EPR微波桥中的脉冲形成单元,用于多个自旋包的自旋激发。通过对植物光系统II中酪氨酸自由基与锰团簇相互作用的PELDOR测量来评价自旋激发的效率。5个不同微波频率辐照的PELDOR光谱的信噪比(S/N)是单一微波频率下的S/N的2.0倍。混合微波频率的使用有效地辐照了宽EPR谱中不同的自旋包,从而提高了宽EPR谱中PELDOR信号的S/N比。在供体Mn^2+存在的情况下,在光系统II中检测到了瞬时EPR信号
英文摘要
In order to investigate quantum teleportation between bio-membrane, radical pairs in photosystem II have been tested. To success the purpose, multiple microwave frequencies in the region of 8.5 -10.5 GHz were applied to spin excitation for pulsed electron paramagnetic resonance (EPR). Five different microwave frequencies were fed to the pulse-forming unit in the EPR microwave bridge and used for spin excitation for multiple spin packets. The efficiency of the spin excitation was evaluated by PELDOR measurements of the interaction between tyrosine radical and the manganese cluster in the plant photosystem II. The signal-to-noise (S/N) ratio of the PELDOR spectrum irradiated by five different microwave frequencies was 2.0 times larger than the S/N from a single microwave frequency. The use of mixed microwave frequencies irradiates the different spin packets in the wide EPR spectrum efficiently, thereby improving the S/N ratio of the PELDOR signal in the broad EPR spectrum. Transient EPR signals was detected in photosystem II in the present of donor Mn^2+
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The electronic structure of S2 state oxygen evolving complex revealed by pulsed ELDOR
脉冲ELDOR揭示S2态氧演化络合物的电子结构
DOI:
--
发表时间:
2012
期刊:
影响因子:
--
作者:
[Mizue Asada, Hiroki Nagashima, Faisal Hammad Mekky Koua, Jian-Ren Shen, Hiroyuki Mino]
通讯作者:
Hiroyuki Mino
Nonselective excitation of pulsed ELDOR using multi-frequency microwaves
使用多频微波非选择性激发脉冲 ELDOR
DOI:
--
发表时间:
2011
期刊:
影响因子:
--
作者:
[Asada, Y. Mutoh, R. Ishiura, M. and Mino H]
通讯作者:
M. and Mino H
複数周波数マイクロ波発生装置を用いた電子電子二重共鳴法における非選択励起
多频微波发生器电子-电子双共振法非选择性激发
DOI:
--
发表时间:
2011
期刊:
影响因子:
--
作者:
[浅田侑希, 武藤梨沙, 石浦正寛, 三野広幸]
通讯作者:
三野広幸
複数周波数のマイクロ波を用いた電子電子二重共鳴法
使用多频微波的电子-电子双共振法
DOI:
--
发表时间:
2010
期刊:
影响因子:
--
作者:
[浅田侑希, 武藤梨沙, 石浦正寛, 三野広幸]
通讯作者:
三野広幸
Protons proximate to Mn cluster in photosystem II are investigated by matrix ENDOR
通过矩阵 ENDOR 研究光系统 II 中 Mn 簇附近的质子
DOI:
--
发表时间:
2012
期刊:
影响因子:
--
作者:
[Hiroki Nagashima, Hiroyuki Mino]
通讯作者:
Hiroyuki Mino
共 15 条
Function of the photo-induced triplet radical pair in the photo-sensor BLUF protein
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批准号:21370069
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项目类别:Grant-in-Aid for Scientific Research (B)
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资助金额:$12.31万
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财政年份:2009
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负责人:MINO Hiroyuki
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依托单位:
海外基金