Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green.

Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green.
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自组装 InGaN 量子点发出绿光的强局域化效应和载流子弛豫动力学

DOI:
10.1186/s11671-015-0772-z
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发表时间:
2015
影响因子:
--
通讯作者:
Zhang BP
Zhang BP
中科院分区:
材料科学3区
文献类型:
--
作者:
Weng GE;Zhao WR;Chen SQ;Akiyama H;Li ZC;Liu JP;Zhang BP

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不同激发功率下的温度依赖性光致发光(PL)证明了金属有机化学气相沉积法生长的自组装InGaN量子点(QDs)具有很强的局部化效应。综合发射强度在30 ~ 160 K范围内逐渐增大,在高激发强度下随着温度的升高而减小,而在低激发强度下这种现象消失。在高激发下,160 K时的发射强度比低温时增强了约40%,内量子效率(IQE)提高了41.1%。提出了一个强局域化模型来描述载流子输运、弛豫和重组的可能过程。利用该模型,可以很好地解释随温度升高的激发功率依赖性发射强度、峰值能量位移和线宽变化的演变。最后,利用双指数模型对不同激发强度下时间分辨PL (TRPL)的双组分衰减进行了观察和分析,从而进一步了解了InGaN量子点中的载流子弛豫动力学。
Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K and then decreases with a further increase in temperature at high excitation intensity, while this phenomenon disappeared at low excitation intensity. Under high excitation, about 40% emission enhancement at 160 K compared to that at low temperature, as well as a higher internal quantum efficiency (IQE) of 41.1%, was observed. A strong localization model is proposed to describe the possible processes of carrier transport, relaxation, and recombination. Using this model, the evolution of excitation-power-dependent emission intensity, shift of peak energy, and linewidth variation with elevating temperature is well explained. Finally, two-component decays of time-resolved PL (TRPL) with various excitation intensities are observed and analyzed with the biexponential model, which enables us to further understand the carrier relaxation dynamics in the InGaN QDs.
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