Waveguiding Nanomaterials: A Path Towards Ultrafast Scintillation Detectors

波导纳米材料：通向超快闪烁探测器的道路

• 批准号: 1708637
• 负责人: Serge Oktyabrsky
• 金额: $ 39.98万
• 依托单位: SUNY Polytechnic Institute
• 依托单位国家: 美国
• 项目类别: Standard Grant
• 财政年份: 2017
• 资助国家: 美国
• 起止时间: 2017-07-15 至 2020-12-31
• 项目状态: 已结题
• 来源: https://www.nsf.gov/awardsearch/showAward?AWD_ID=1708637&HistoricalAwards=false
• 关键词: Waveguiding; Nanomaterials; Path; Towards; Ultrafast

Nontechnical Description: This project addresses science and technology of a new materials system comprising nanoscale islands - quantum dots - embedded in a thin semiconductor film. The electronic and optical properties of the materials are designed to enable ultrafast detection of x-rays and energetic quantum particles. The key element of this sensing material is a light-emitting quantum dot ensemble capable of converting energy from incoming x-rays into infrared light. This type of material performance, known as scintillation, is carried out with unsurpassed energetic yield and speed, thus providing a long-expected solution for key technological applications. Such ultrafast x-ray detection is essential for implementing low-dose x-ray three-dimensional medical imaging, as in computer or positron-emission tomography (PET), as well as for improving accuracy and turnaround time in nuclear systems security. The project enables technology development and commercialization, potentially facilitating the emergence of higher quality medical and defense instrumentation at reduced cost. The educational component of the project includes direct support of a graduate student research assistant towards a Ph.D. in nanoscale engineering, hands-on training of undergraduate students, launching a new optical nanomaterials laboratory segment for K-12 students, and training of science teachers within the educational College infrastructure. Technical Description: The relatively weak existing material interactions at high energies lead to a fundamental challenge for picosecond-scale timing of energetic particles and photons. A large-volume scintillation medium coupled to a small and fast photodetector is the preferable approach to remedy this limitation, where the time response is limited by the excitation transfer and emission, as well as the optical transit time. This project develops a new scientific approach and technology for a scintillation material using quantum dots as nano-engineered emission centers capable of providing unsurpassed speed and light yield, additionally exploring detector integration in order to test the performance benefits. While the concept is not material-specific, the current technology level and the required device properties favor self-assembled InAs quantum dots (QDs) embedded in a GaAs waveguide as the test material system. The project includes a modeling component, engineering and fabrication of QD waveguides with an integrated photodetector, and assessment of time and energy resolution. This study paves a path for enabling reduced radiation doses in medical 3D imaging/tomography applications, improving spectroscopic accuracy in nuclear security, and enhancing particle identification capabilities in high-energy physics experiments. The project enables technology development and commercialization efforts, promotion of nanotechnology to the broader public, additionally enriching the College outreach infrastructure.

非技术描述：该项目涉及一种新材料系统的科学和技术，该系统包括嵌入薄半导体薄膜中的纳米级岛-量子点。这些材料的电子和光学特性旨在实现X射线和高能量子粒子的超快检测。这种传感材料的关键元素是一种发光量子点集合体，能够将入射X射线的能量转换为红外光。这种类型的材料性能，称为闪烁，以无与伦比的能量产量和速度进行，从而为关键技术应用提供了长期期待的解决方案。这种超快X射线探测对于实现低剂量X射线三维医学成像（如在计算机或正电子发射断层扫描（PET）中）以及对于提高核系统安全的准确性和周转时间至关重要。该项目使技术开发和商业化成为可能，从而可能以更低的成本促进更高质量的医疗和国防仪器的出现。该项目的教育部分包括直接支持研究生研究助理攻读博士学位在纳米级工程，动手培训的本科生，推出一个新的光学纳米材料实验室部分的K-12学生，和培训科学教师的教育学院基础设施。 技术说明：在高能量下相对较弱的现有材料相互作用导致高能粒子和光子的皮秒尺度计时的根本挑战。耦合到小而快的光电探测器的大体积闪烁介质是补救这种限制的优选方法，其中时间响应受到激发转移和发射以及光学渡越时间的限制。该项目开发了一种新的科学方法和技术，用于使用量子点作为纳米工程发射中心的闪烁材料，能够提供无与伦比的速度和光产量，此外还探索了探测器集成，以测试性能优势。虽然这个概念不是特定的材料，目前的技术水平和所需的设备特性有利于自组装InAs量子点（QD）嵌入在GaAs波导作为测试材料系统。该项目包括一个建模组件，工程和制造的QD波导与集成光电探测器，时间和能量分辨率的评估。这项研究为降低医学3D成像/断层扫描应用中的辐射剂量，提高核安全中的光谱准确性以及增强高能物理实验中的粒子识别能力铺平了道路。该项目使技术开发和商业化的努力，促进纳米技术更广泛的公众，另外丰富学院的外联基础设施。

项目成果

Parameters of fast and high-yield InAs/GaAs quantum dot semiconductor scintillator

快速高产InAs/GaAs量子点半导体闪烁体参数

• DOI: 10.1557/s43580-021-00019-y
• 发表时间: 2021
• 期刊: MRS Advances
• 影响因子: 0.8
• 作者: Minns, A.;Dropiewski, K.;Yakimov, M.;Tokranov, V.;Hedges, M.;Murat, P.;Oktyabrsky, S.
• 通讯作者: Oktyabrsky, S.

Ultrafast InAs Quantum Dot Scintillation Detector

超快 InAs 量子点闪烁探测器

• 发表时间: 2019
• 期刊: 235th ECS Meeting
• 作者: K. Dropiewski, A.Minns

Ultrafast Waveguiding Quantum Dot Scintillation Detector

超快波导量子点闪烁探测器

• DOI: 10.1016/j.nima.2018.10.150
• 发表时间: 2018
• 期刊: Detectors and Associated Equipment
• 作者: Dropiewski, K.;Minns, A.;Yakimov, M.;Tokranov, V.;Murat, P.;Oktyabrsky, S.
• 通讯作者: Oktyabrsky, S.

Optical Properties of InAs Quantum Dots/GaAs Waveguides for Ultra-fast Scintillators

用于超快闪烁体的 InAs 量子点/GaAs 波导的光学特性

• DOI: 10.1016/j.jlumin.2019.116952
• 发表时间: 2020
• 期刊: Journal of Luminescence
• 影响因子: 3.6
• 作者: Dropiewski, K.;Minns, A.;Yakimov, M.;Tokranov, V.;Murat, P.;Oktyabrsky, S.
• 通讯作者: Oktyabrsky, S.

Optimization of InAs Quantum Dots for Scintillation Applications

用于闪烁应用的 InAs 量子点优化

• 发表时间: 2018
• 期刊: The 34th North American Conference on Molecular Beam Epitaxy (NAMBE 2018
• 作者: M. Yakimov, V. Tokranov