Enhancing Quantum Emissions from Atomically Thin Semiconductors with Metasurfaces

利用超表面增强原子薄半导体的量子发射

• 批准号: 2130552
• 负责人: Xiaoqin Li
• 金额: $ 35.12万
• 依托单位: University of Texas at Austin
• 依托单位国家: 美国
• 项目类别: Standard Grant
• 财政年份: 2021
• 资助国家: 美国
• 起止时间: 2021-09-01 至 2024-08-31
• 项目状态: 已结题
• 来源: https://www.nsf.gov/awardsearch/showAward?AWD_ID=2130552&HistoricalAwards=false
• 关键词: Enhancing; Quantum; Emissions; Atomically; Thin

Atomically thin semiconductors refer to materials that are only one or a few unit-cell thick. They can be created by peeling off layers from van der Waals materials that consist of weakly bound two-dimensional layers or grown using chemical processes that have already been developed in the semiconductor industry. Metasurfaces refer to a class of flat optics that include engineered unit cells smaller than the wavelength of light. Integrating atomically thin materials with metasurfaces brings exciting new opportunities for quantum technology. As an example, an array of quantum emitters that generate one photon at a time can be used for enhancing community security. In this project, metasurface engineering strategies will be designed and implemented to broadcast such quantum emitters such as the signal is brighter due to quantum collective phenomena with better-controlled emission direction and efficiency. The proposed projects will provide excellent training opportunities for both graduate and undergraduate students and prepare a workforce to compete globally in quantum technologies.Technical:When two atomically thin van der Waals layers are vertically stacked together, the atomic alignment between the layers exhibits periodical variations, leading to a new type of in-plane superlattices known as the moiré superlattices. They represent one of the most exciting developments of photonic materials that have just emerged in the last few years. In this program, the quantum emissions from transition metal dichalcogenides moire superlattice will be enhanced using various metasurfaces, charting new territories of hybrid photonic platforms. Specific goals include (i) broadcasting an array of quantum emitters hosted in moire superlattices using nano-antennas; (ii) selective excitation of valley polarized emitters using chiral metasurfaces; (iii) realizing collective quantum emission with zero-index metasurfaces. The proposed projects explore new types of quantum photonic materials with the potential to address long-standing challenges of solid-state quantum emitters. The program will integrate undergraduate and graduate education with cutting-edge research activities.This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.

原子薄型半导体指的是只有一个或几个单位电池厚度的材料。它们可以通过剥离由弱结合的二维层组成的范德华材料的层来产生，或者使用半导体行业已经开发的化学工艺来生长。亚表面指的是一类平面光学器件，其中包括小于光波长的工程单元单元。将原子薄材料与超表面相结合为量子技术带来了令人兴奋的新机遇。例如，一次产生一个光子的量子发射器阵列可以用于增强社区安全。在本项目中，将设计和实现超表面工程策略，以更好地控制发射方向和效率，以广播由于量子集体现象而导致的信号更亮等量子发射体。拟议的项目将为研究生和本科生提供极好的培训机会，并为量子技术领域的全球竞争培养一支队伍。技术：当两个原子薄的范德华层垂直堆叠在一起时，层之间的原子排列呈现周期性变化，从而产生一种新型的面内超晶格，称为莫尔超晶格。它们代表了过去几年刚刚出现的光子材料最令人兴奋的发展之一。在这个项目中，过渡金属二盐基化物莫尔超晶格的量子发射将使用各种亚表面来增强，绘制出混合光子平台的新领域。具体目标包括：(I)利用纳米天线在莫尔超晶格中传播一系列量子发射体；(Ii)使用手性亚表面选择性激发谷极化发射体；(Iii)利用零折射率亚表面实现集体量子发射。拟议的项目探索新型量子光子材料，有可能解决固态量子发射器长期存在的挑战。该计划将本科生和研究生教育与尖端研究活动相结合。该奖项反映了NSF的法定使命，并通过使用基金会的智力优势和更广泛的影响审查标准进行评估，被认为值得支持。

项目成果

Fermi Pressure and Coulomb Repulsion Driven Rapid Hot Plasma Expansion in a van der Waals Heterostructure

• DOI: 10.1021/acs.nanolett.3c00678
• 发表时间: 2023-05-08
• 期刊: NANO LETTERS
• 影响因子: 10.8
• 作者: Choi, Junho;Embley, Jacob;Huang, Libai
• 通讯作者: Huang, Libai

Anisotropic Excitons Reveal Local Spin Chain Directions in a van der Waals Antiferromagnet

• DOI: 10.1002/adma.202206585
• 发表时间: 2023-02
• 期刊: Advanced Materials
• 影响因子: 29.4
• 作者: Dong Seob Kim;Di Huang;Chunhao Guo;Kejun Li;D. Rocca;Frank Y. Gao;Jeongheon Choe;David Lujan;Ting-Hsuan Wu;Kung‐Hsuan Lin;E. Baldini;Li Yang;Shivani Sharma;R. Kalaivanan;R. Sankar;Shang-Fan Lee;Y. Ping;Xiaoqin Li