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Post-Combustion Carbon Capture Using MOFs: Materials and Process Development

使用 MOF 进行燃烧后碳捕获：材料和工艺开发

基本信息

批准号：
EP/L021064/1
负责人：
Stefano Brandani
金额：
$ 25.19万
依托单位：
University of Edinburgh
依托单位国家：
英国
项目类别：
Research Grant
财政年份：
2014
资助国家：
英国
起止时间：
2014 至无数据
项目状态：
已结题

来源：
https://gtr.ukri.org/projects?ref=EP%2FL021064%2F1
关键词：
Post Combustion Carbon Capture Using

项目摘要

The proposal aims to develop an international collaborative research programme under Topic 4 of the FENCO-NET call: New innovative CO2capture technologies. The specific issues addressed in the proposal are:1. Overall evaluation of new innovative CO2 capture processes based on Metal Organic Framework (MOF) materials;2. To synthesise (scale-up to kg quantities), characterise,, formulate and evaluate selected MOFs for vacuum swing (VSA) post-combustion capture;3. To investigate and address adsorbent stability and efficiency in post-combustion carbon capture processes;4. To investigate and model mass and heat transfer kinetics to enable accurate dynamic process simulations needed for the optimization of thecarbon capture units with respect to energy efficiency and operational and capital costs.The FENCO-NET call gives the unique opportunity of coordinating the significant research efforts in the partner institutions. SINTEF has thecapability of preparing advanced MOFs which can also be scaled-up to produce formed materials for bench scale process testing. The UoE hasdeveloped new rapid screening techniques, specifically for post-combustion carbon capture and the close collaboration with SINTEF will acceleratefurther developments and provide essential stability data to direct novel material synthesis. Significant advances in this field can only be achieved ifmaterial and process development are combined. CERTH brings significant expertise in Vacuum Swing Adsorption (VSA) modelling, simulation, designand optimization and both the UoE and SINTEF have the capability of evaluating the integration of the novel carbon capture systems in power plants.

该提案旨在在FENCO-Net呼吁的主题4：新的创新性二氧化碳捕获技术下制定一项国际合作研究方案。建议中涉及的具体问题是：1.基于金属有机框架(MOF)材料的新的创新二氧化碳捕获工艺的总体评估；2.合成(放大到千克量)、表征、配制和评估选定的金属有机骨架燃烧后捕获(VSA)；3.调查和解决燃烧后碳捕获过程中的吸附剂稳定性和效率问题；4.对传质和传热动力学进行研究和建模，以实现在能源效率以及运营和资本成本方面优化碳捕获装置所需的准确动态过程模拟。FENCO-NET呼吁为协调合作机构的重大研究工作提供了独特的机会。SINTEF有能力制备先进的MOF，这些MOF也可以放大生产成型材料，用于小试工艺试验。UOE开发了新的快速筛选技术，专门用于燃烧后碳捕获，与SINTEF的密切合作将加快进一步的开发，并为指导新材料合成提供必要的稳定性数据。只有在材料和工艺开发相结合的情况下，才能在这一领域取得重大进展。CERTH在真空摆动吸附(VSA)建模、模拟、设计和优化方面拥有丰富的专业知识，UOE和SINTEF都有能力评估发电厂中新型碳捕获系统的集成。