Aersol and Clouds - ACID-PRUF

气溶胶和云 - ACID-PRUF

基本信息

批准号：
NE/I020008/1
负责人：
Paul Monks
金额：
$ 20.9万
依托单位：
University of Leicester
依托单位国家：
英国
项目类别：
Research Grant
财政年份：
2011
资助国家：
英国
起止时间：
2011 至无数据
项目状态：
已结题

来源：
https://gtr.ukri.org/projects?ref=NE%2FI020008%2F1
关键词：
Aersol Clouds ACID PRUF

项目摘要

Aerosol particles act as sites for cloud droplet and ice particle formation. Cloud properties can be perturbed through the addition of aerosol particles into the atmosphere from anthropogenic and natural processes. This addition influences cloud microphysical properties, and subsequently affects cloud dynamics and thermodynamics, and the way the cloud interacts with radiation. The Earth's radiation budget is very greatly affected by clouds, and human-induced changes to the particle loading affecting them, known as indirect effects, are large and highly uncertain. A large part of this uncertainty is the result of poor knowledge of the fundamental aerosol and cloud properties and processes, leading to their poor representation in models. A programme of research is proposed here to i) directly investigate these processes in the laboratory, ii) evaluate the sensitivity of climate relevant parameters to the studied processes, iii) interpret the laboratory studies with detailed model investigations and iv) to incorporate and test new descriptions of the studied processes in cloud-scale and, where possible, global scale models. The programme will thereby reduce the uncertainty in estimates of radiative forcing and climate feedbacks relating to aerosol and cloud processes. The studies are split into those affecting warm clouds (those containing only liquid droplets) and those affecting clouds containing ice particles. The programme brings together an interdisciplinary team of researchers with expertise in 'warm' and 'cold' cloud and aerosol processes combining laboratory and multiscale modelling activities to deliver the improved predictive capability. The 'warm' laboratory work focuses on two major aspects i) the rate at which water is taken up by growing aerosol particles as they become cloud droplets (or 'activate) and ii) the ability of aerosol particles of various compositions to act as seeds for cloud droplets. These studies use a number of techniques including single particle optical levitation and investigations in a large photochemical chamber coupled to a large number of chemical and physical probes of ensembles of particles formed in simulated atmospheric chemical processes. The 'cold' work uses a similar coupling of a large, well-instrumented cloud chamber experiments and single particle levitation studies. The chambers used in both aspects will be coupled to investigate the impacts of aerosol transformation conditions on warm and cold cloud formation, using the instrumental payload from both chambers. A range of detailed models will be used to explicitly describe the processes by which aerosol particles interact with increasing relative humidity and reducing temperature to form cloud droplet and ice crystals and to their properties. The processes and properties will be represented in dynamical frameworks to predict the interactions between aerosols and clouds and their radiative effects at cloud resolving scales and radiative forcing of some of the investigated properties on global radiative forcing and feedbacks. The sensitivity of climate relevant parameters to the fundamental parameters investigated in the laboratory programme and their improved quantification will be evaluated using a simplified model 'emulator'.

气溶胶颗粒充当云滴和冰颗粒形成的位置。通过通过人为和自然过程将气溶胶颗粒添加到大气中，可以通过将气溶胶颗粒添加到大气中受到干扰。此添加影响云微物理特性，并随后影响云动力学和热力学，以及云与辐射相互作用的方式。地球的辐射预算极大地受到云的影响，人类引起的影响粒子负荷的变化（称为间接影响）是大而高度不确定的。这种不确定性的很大一部分是对基本气溶胶和云特性和过程的知识不足的结果，导致它们在模型中的代表性不佳。这里提出了一项研究计划。该计划将减少与气溶胶和云过程有关的辐射强迫和气候反馈的估计值的不确定性。研究分为影响温暖云（仅包含液滴的云）和影响含有冰颗粒的云的那些。该计划汇集了一个跨学科的研究人员团队，具有“温暖”和“冷”云和气溶胶过程的专业知识，结合了实验室和多尺度建模活动，以提供改进的预测能力。 “温暖”实验室工作的重点是两个主要方面i）在气溶胶颗粒变成云液滴（或“激活）和ii）各种组合物的气溶胶颗粒充当云滴的种子的能力时，将水吸收水的速率。这些研究使用了许多技术，包括单个粒子光悬浮和在大型光化学室中进行的研究，并与在模拟大气化学过程中形成的颗粒组合的大量化学和物理探针结合在一起。 “冷”工作使用了大型，备受启发的云腔实验和单个颗粒悬浮研究的类似耦合。在这两个方面使用的室将使用来自两个腔室的仪器有效载荷研究气溶胶转化条件对温暖和冷云形成的影响。一系列详细的模型将用于明确描述气溶胶颗粒与增加的相对湿度和降低温度相互作用以形成云滴和冰晶以及其性能的过程。这些过程和属性将在动态框架中表示，以预测气溶胶与云之间的相互作用及其在云解析尺度下的辐射效应，并在全球辐射强迫和反馈中对某些研究的特性进行辐射强迫。气候相关参数对实验室计划中研究的基本参数及其改进的定量的敏感性将使用简化的模型“模拟器”评估。

项目成果

期刊论文数量（10）

专著数量（0）

科研奖励数量（0）

会议论文数量（0）

专利数量（0）

Mapping gas-phase organic reactivity and concomitant secondary organic aerosol formation: chemometric dimension reduction techniques for the deconvolution of complex atmospheric data sets

DOI：
10.5194/acp-15-8077-2015
发表时间：
2015-07
期刊：
Atmospheric Chemistry and Physics
影响因子：
6.3
作者：
K. Wyche;P. Monks;K. Smallbone;J. Hamilton;M. Alfarra;A. Rickard;G. Mcfiggans;M. Jenkin;W. Bloss;Annette C Ryan;C. Hewitt;A. MacKenzie
通讯作者：
K. Wyche;P. Monks;K. Smallbone;J. Hamilton;M. Alfarra;A. Rickard;G. Mcfiggans;M. Jenkin;W. Bloss;Annette C Ryan;C. Hewitt;A. MacKenzie

Water uptake is independent of the inferred composition of secondary aerosols derived from multiple biogenic VOCs

DOI：
10.5194/acp-13-11769-2013
发表时间：
2013-01-01
期刊：
ATMOSPHERIC CHEMISTRY AND PHYSICS
影响因子：
6.3
作者：
Alfarra, M. R.;Good, N.;McFiggans, G.
通讯作者：
McFiggans, G.

Online and offline mass spectrometric study of the impact of oxidation and ageing on glyoxal chemistry and uptake onto ammonium sulfate aerosols.

DOI：
10.1039/c3fd00051f
发表时间：
2013-12
期刊：
Faraday discussions
影响因子：
3.4
作者：
J. Hamilton;M. Baeza_Romero;E. Finessi;R. Andrew;Rickard;R. Healy;S. Peppe;T. J. Adams;S. M
通讯作者：
J. Hamilton;M. Baeza_Romero;E. Finessi;R. Andrew;Rickard;R. Healy;S. Peppe;T. J. Adams;S. M

New Directions: Fundamentals of atmospheric chemistry: Keeping a three-legged stool balanced