Functional covalent triazine frameworks for catalysis and energy storage applications

用于催化和储能应用的功能性共价三嗪框架

基本信息

  • 批准号:
    RGPIN-2020-05546
  • 负责人:
  • 金额:
    $ 2.84万
  • 依托单位:
  • 依托单位国家:
    加拿大
  • 项目类别:
    Discovery Grants Program - Individual
  • 财政年份:
    2020
  • 资助国家:
    加拿大
  • 起止时间:
    2020-01-01 至 2021-12-31
  • 项目状态:
    已结题

项目摘要

Polymers with intrinsic porosity in both the micro- and macroscopic scale have aroused enormous research interest for a variety of functional applications because of their unique structures and resulting superior properties. Covalent triazine frameworks (CTFs), synthesized often by trimerization of aromatic nitriles, are an exciting class of porous polymers with tunable structure, high chemical stability, and rich heteroatom contents, which facilitate their emerging applications in various fields. The overall objective of this proposed DG research is to develop and design a novel range of functional CTFs of tunable well-defined structures/functionalities and superior performance properties for applications in catalysis and energy storage areas. Three specific projects are defined: (1) developing CTFs as novel 3D macromolecular ligands for Pd-based olefin polymerization catalysts; (2) developing heterogeneous functional CTF-supported Pd nanocatalysts for semi-hydrogenation of alkynes; (3) developing CTF nanocomposite anode materials for lithium-ion batteries. The proposed research is highly multidisciplinary in nature and combines diverse disciplines including polymer chemistry and physics, nanotechnology, materials science, catalysis, and energy storage techniques. It is expected that this research will lead to a novel class of CTF materials of tailored structures and superior performance properties, which may find value-added applications in catalysis and energy storage areas. The fundamental knowledge to be generated in this research will also contribute significantly to the design and synthesis of porous polymer materials, catalysis materials, and energy storage materials, and broaden the understanding of the structure-performance relationships. Moreover, the proposed research will also offer valuable opportunities for the training of next-generation researchers for Canadian universities, industries, and government research laboratories.
在微观和宏观尺度上具有固有孔隙率的聚合物由于其独特的结构和由此产生的上级性能而在各种功能应用中引起了巨大的研究兴趣。共价三嗪骨架(CTFs)是一类结构可调、化学稳定性高、杂原子含量丰富的多孔聚合物,其应用前景广阔。该DG研究的总体目标是开发和设计一系列新的功能性CTF,其具有可调的明确结构/功能和上级性能特性,可用于催化和储能领域。确定了三个具体项目:(1)开发CTF作为新型三维大分子配体用于Pd基烯烃聚合催化剂;(2)开发用于炔半加氢的多相功能CTF负载Pd纳米催化剂;(3)开发用于锂离子电池的CTF纳米复合负极材料。 拟议的研究是高度多学科的性质,并结合了不同的学科,包括聚合物化学和物理,纳米技术,材料科学,催化和储能技术。 预计这项研究将导致一种新型的CTF材料的定制结构和上级性能,这可能会发现在催化和能量存储领域的增值应用。本研究所产生的基础知识也将对多孔聚合物材料、催化材料和储能材料的设计和合成做出重要贡献,并拓宽对结构-性能关系的理解。此外,拟议的研究还将为加拿大大学、工业和政府研究实验室培训下一代研究人员提供宝贵的机会。

项目成果

期刊论文数量(0)
专著数量(0)
科研奖励数量(0)
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Ye, Zhibin其他文献

The association of urinary prostaglandins with uric acid in hyperuricemia patients.
  • DOI:
    10.1186/s12882-022-02928-y
  • 发表时间:
    2022-09-03
  • 期刊:
  • 影响因子:
    2.3
  • 作者:
    Lin, Huagang;Xu, Ying;Zheng, Yuqi;Wu, Deping;Ye, Zhibin;Xiao, Jing
  • 通讯作者:
    Xiao, Jing
Multimode tunable terahertz absorber based on a quarter graphene disk structure
  • DOI:
    10.1016/j.rinp.2023.106420
  • 发表时间:
    2023-04-07
  • 期刊:
  • 影响因子:
    5.3
  • 作者:
    Ye, Zhibin;Wu, Pinghui;Wu, Fei
  • 通讯作者:
    Wu, Fei
Sulfonated polyaryletherketone with pendant benzimidazole groups for proton exchange membranes
  • DOI:
    10.1016/j.memsci.2019.117626
  • 发表时间:
    2020-03-01
  • 期刊:
  • 影响因子:
    9.5
  • 作者:
    Liang, Jun;Ge, Jiao;Ye, Zhibin
  • 通讯作者:
    Ye, Zhibin
Clinical classification of hyperuricemia in patients with chronic kidney disease
  • DOI:
    10.1007/s11255-020-02754-x
  • 发表时间:
    2021-01-02
  • 期刊:
  • 影响因子:
    2
  • 作者:
    Li, Fengqin;Guo, Hui;Ye, Zhibin
  • 通讯作者:
    Ye, Zhibin
Efficacy of different urinary uric acid indicators in patients with chronic kidney disease
  • DOI:
    10.1186/s12882-020-01953-z
  • 发表时间:
    2020-07-22
  • 期刊:
  • 影响因子:
    2.3
  • 作者:
    Guan, Haochen;Zheng, Yuqi;Ye, Zhibin
  • 通讯作者:
    Ye, Zhibin

Ye, Zhibin的其他文献

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{{ truncateString('Ye, Zhibin', 18)}}的其他基金

Functional covalent triazine frameworks for catalysis and energy storage applications
用于催化和储能应用的功能性共价三嗪框架
  • 批准号:
    RGPIN-2020-05546
  • 财政年份:
    2022
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Discovery Grants Program - Individual
Functional covalent triazine frameworks for catalysis and energy storage applications
用于催化和储能应用的功能性共价三嗪框架
  • 批准号:
    RGPIN-2020-05546
  • 财政年份:
    2021
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Discovery Grants Program - Individual
Developing semicrystalline star polyethylenes and advanced polyethylene ionomers
开发半结晶星形聚乙烯和先进的聚乙烯离聚物
  • 批准号:
    RGPIN-2015-03815
  • 财政年份:
    2019
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Discovery Grants Program - Individual
Polymer Nanomaterials
高分子纳米材料
  • 批准号:
    1000230723-2014
  • 财政年份:
    2018
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Canada Research Chairs
Developing semicrystalline star polyethylenes and advanced polyethylene ionomers
开发半结晶星形聚乙烯和先进的聚乙烯离聚物
  • 批准号:
    RGPIN-2015-03815
  • 财政年份:
    2018
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Discovery Grants Program - Individual
Lignin-Polymer Composite Materials: Production Process Optimization and Product Performance Evaluation
木质素-聚合物复合材料:生产工艺优化及产品性能评价
  • 批准号:
    536687-2018
  • 财政年份:
    2018
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Engage Plus Grants Program
Developing semicrystalline star polyethylenes and advanced polyethylene ionomers
开发半结晶星形聚乙烯和先进的聚乙烯离聚物
  • 批准号:
    477901-2015
  • 财政年份:
    2017
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Discovery Grants Program - Accelerator Supplements
Lignin-Polyethylene Composite Materials: Production Process Optimization and Performance Evaluation
木质素-聚乙烯复合材料:生产工艺优化及性能评价
  • 批准号:
    517418-2017
  • 财政年份:
    2017
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Engage Grants Program
Developing semicrystalline star polyethylenes and advanced polyethylene ionomers
开发半结晶星形聚乙烯和先进的聚乙烯离聚物
  • 批准号:
    RGPIN-2015-03815
  • 财政年份:
    2017
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Discovery Grants Program - Individual
Polymer Nanomaterials
高分子纳米材料
  • 批准号:
    1000230723-2014
  • 财政年份:
    2017
  • 资助金额:
    $ 2.84万
  • 项目类别:
    Canada Research Chairs

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