Terahertz Electron Hole Recollisions

太赫兹电子空穴碰撞

基本信息

  • 批准号:
    1405964
  • 负责人:
  • 金额:
    $ 56.5万
  • 依托单位:
  • 依托单位国家:
    美国
  • 项目类别:
    Standard Grant
  • 财政年份:
    2014
  • 资助国家:
    美国
  • 起止时间:
    2014-07-01 至 2017-06-30
  • 项目状态:
    已结题

项目摘要

Non-technical abstract:In high-energy physics, the structure of matter is explored by accelerating and colliding elementary particles like electrons and protons. In condensed matter physics, the fundamental excitations are called quasi-particles. The most familiar quasi-particles are electrons and holes in semiconductors, which can be created for example in a solar photovoltaic cell - by light with a sufficiently short wavelength. In this project, electrons and holes will be created by a weak near-infrared laser with a wavelength slightly longer than is visible to the human eye, and will be made to accelerate and then recollide with one another by a very strong electric field oscillating nearly 1 trillion times per second (1 Terahertz). The recollision process will be studied by analyzing the spectrum (which wavelengths are present) in the transmitted near-infrared light. This spectrum has been shown to contain up to 18 separate nearinfrared wavelengths, or sidebands, in addition to the wavelength of the near-infrared laser that creates electron-hole pairs. This research will elucidate how much quasiparticles can be accelerated without being disturbed by defects or the motion of atoms in their host material. The proposed research may lead to faster and more energy efficient optical communications and internet, and improved optical clocks that are necessary in the global positioning system. This project will support the training of two Ph. D. students, who will learn a variety of skills that are critical to preserving U. S. competitiveness in the high-technology sector.Technical abstract:High-order sideband generation, a new phenomenon in the interaction of light with matter, was recently discovered in the PI's research group. A relatively weak, continuous-wave near-infrared (NIR) laser at frequency ~350 THz, and an intense laser at frequency ~0.5 THz are incident on a thin film of semiconductor. A comb of equally-spaced sidebands is emitted, with sharp lines at sideband frequency = NIR frequency + 2n THz frequency, where n is an integer. Combs with up to 14 sidebands (order up to 2*14=28) above NIR frequency have been observed. The high-order sidebands can be understood in terms of a semiclassical model similar to one that was first introduced to explain high-order harmonic generation, an analogous phenomenon that occurs for atoms in intense laser fields. In high-order-sideband generation (HSG), the NIR laser creates excitons, bound electron-hole pairs. The strong THz field ionizes the excitons, and accelerates the resulting electron and hole into a large-amplitude oscillation. When the electron and hole recollide, the excess kinetic energy is carried off in sidebands above the NIR frequency. This project will explore the onset of high-order sideband generation, whether there is a fundamental limit on the number of observable sidebands, whether the shape of the sideband spectrum can be controlled, and whether, in the case of a circularly-polarized terahertz field, the polarization of the near-ir radiation is rotated. By exploring the limits of HSG, the proposed research will elucidate potential applications of HSG to electro-optic technologies ranging from optical communications to optical clocks. This project will support the training of two Ph.D. students, who will learn a variety of skills including near-ir and terahertz optics, cryogenics, electronics, computer programming, and mechanical and optomechanical design.
非技术摘要:在高能物理学中,物质的结构是通过加速和碰撞基本粒子如电子和质子来探索的。在凝聚态物理学中,基本的激发被称为准粒子。最熟悉的准粒子是半导体中的电子和空穴,它们可以在太阳能光伏电池中产生-通过波长足够短的光。在这个项目中,电子和空穴将由波长略长于人眼可见的弱近红外激光产生,并将通过每秒振荡近1万亿次(1太赫兹)的非常强的电场加速,然后相互碰撞。将通过分析透射近红外光中的光谱(存在哪些波长)来研究分解过程。该光谱已被证明包含多达18个独立的近红外波长或边带,除了产生电子空穴对的近红外激光的波长之外。这项研究将阐明在不受缺陷或宿主材料中原子运动干扰的情况下,准粒子可以被加速多少。拟议的研究可能会导致更快,更节能的光通信和互联网,以及全球定位系统所需的改进的光学时钟。该项目将支持培养两名博士。学生,谁将学习各种技能,是至关重要的,以保持美国。S.技术摘要:PI的研究小组最近发现了光与物质相互作用中的一种新现象--高阶边带的产生。一个相对较弱的,连续波近红外(NIR)激光频率约350太赫兹,和一个强激光频率约0.5太赫兹入射到半导体薄膜。发射等间隔边带的梳状,边带频率= NIR频率+2n THz频率处具有尖锐线,其中n是整数。已经观察到在NIR频率以上具有多达14个边带(阶数高达2*14=28)的梳。高阶边带可以用半经典模型来理解,该模型类似于首次引入来解释高次谐波产生的模型,高次谐波产生是强激光场中原子发生的类似现象。在高阶边带产生(HSG)中,NIR激光器产生激子,束缚电子-空穴对。强太赫兹场使激子电离,并将产生的电子和空穴加速成大振幅振荡。当电子和空穴相互作用时,多余的动能在高于NIR频率的边带中被带走。本计画将探讨高阶边带产生的开始,可观测边带的数量是否有基本限制,边带频谱的形状是否可以控制,以及在圆极化太赫兹场的情形下,近红外辐射的极化是否会旋转。通过探索HSG的局限性,拟议的研究将阐明HSG在从光通信到光钟的电光技术中的潜在应用。该项目将支持培养两名博士。学生将学习各种技能,包括近红外和太赫兹光学、低温学、电子学、计算机编程以及机械和光学机械设计。

项目成果

期刊论文数量(2)
专著数量(0)
科研奖励数量(0)
会议论文数量(0)
专利数量(0)
Dynamical Birefringence: Electron-Hole Recollisions as Probes of Berry Curvature
  • DOI:
    10.1103/physrevx.7.041042
  • 发表时间:
    2017-11-21
  • 期刊:
  • 影响因子:
    12.5
  • 作者:
    Banks, Hunter B.;Wu, Qile;Sherwin, Mark S.
  • 通讯作者:
    Sherwin, Mark S.
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Mark Sherwin其他文献

Terahertz power
太赫兹功率
  • DOI:
    10.1038/420131a
  • 发表时间:
    2002-11-14
  • 期刊:
  • 影响因子:
    48.500
  • 作者:
    Mark Sherwin
  • 通讯作者:
    Mark Sherwin

Mark Sherwin的其他文献

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{{ truncateString('Mark Sherwin', 18)}}的其他基金

Bloch wave interferometry in semiconductors and correlated insulators
半导体和相关绝缘体中的布洛赫波干涉测量
  • 批准号:
    2333941
  • 财政年份:
    2024
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Standard Grant
MRI: Development of an Agile Free-Electron-Laser-Powered Pulsed Electron Magnetic Resonance (FEL-EMR) Spectrometer
MRI:开发敏捷自由电子激光驱动脉冲电子磁共振 (FEL-EMR) 能谱仪
  • 批准号:
    2117994
  • 财政年份:
    2021
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Standard Grant
Colliding quasiparticles to reconstruct their effective Hamiltonians
碰撞准粒子重建其有效哈密顿量
  • 批准号:
    2004995
  • 财政年份:
    2020
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Continuing Grant
Triggered functional dynamics of proteins in biomimetic environments by time-resolved electron paramagnetic resonance at very high magnetic fields
通过极高磁场下的时间分辨电子顺磁共振触发仿生环境中蛋白质的功能动力学
  • 批准号:
    2025860
  • 财政年份:
    2020
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Standard Grant
Terahertz Recollisions
太赫兹再碰撞
  • 批准号:
    1710639
  • 财政年份:
    2017
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Continuing Grant
MRI: Development of a single-mode terahertz free electron lasers for research in materials, physics, chemistry and biology
MRI:开发单模太赫兹自由电子激光器,用于材料、物理、化学和生物学研究
  • 批准号:
    1626681
  • 财政年份:
    2016
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Standard Grant
Time-resolved conformational changes of proteins by very high frequency Gd3+ EPR
通过甚高频 Gd3 EPR 实现蛋白质的时间分辨构象变化
  • 批准号:
    1617025
  • 财政年份:
    2016
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Standard Grant
Robust Gd3+ -based spin labels for structural studies of membrane proteins
用于膜蛋白结构研究的基于 Gd3 的稳健自旋标签
  • 批准号:
    1244651
  • 财政年份:
    2013
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Continuing Grant
MRI: Development of a Free-Electron Laser for Ultrafast Pulsed Electron Paramagnetic Resonance
MRI:开发用于超快脉冲电子顺磁共振的自由电子激光器
  • 批准号:
    1126894
  • 财政年份:
    2011
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Standard Grant
Quantum Coherence and Dynamical Instability in Quantum Wells Driven by Intense Terahertz Fields.
强太赫兹场驱动的量子井中的量子相干性和动态不稳定性。
  • 批准号:
    1006603
  • 财政年份:
    2010
  • 资助金额:
    $ 56.5万
  • 项目类别:
    Continuing Grant

相似国自然基金

Muon--electron转换过程的实验研究
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