Synthesis, Properties and Structure-Function Relationships in Ferecrystals: New Compounds Composed of Stacked 2D Layers with Designed Nanoarchitecture

Ferecrystals 的合成、性能和结构功能关系:具有设计纳米结构的堆叠二维层组成的新化合物

基本信息

  • 批准号:
    1710214
  • 负责人:
  • 金额:
    $ 45万
  • 依托单位:
  • 依托单位国家:
    美国
  • 项目类别:
    Standard Grant
  • 财政年份:
    2017
  • 资助国家:
    美国
  • 起止时间:
    2017-08-01 至 2020-07-31
  • 项目状态:
    已结题

项目摘要

Non-technical Abstract:A grand challenge in materials research is the preparation of novel compounds with designed properties. The ability to create stable layered materials with complicated layering schemes provides an unprecedented ability to probe the interplay between structure, composition, and physical properties of the constituents. This research produces a rich collection of new materials with diverse and highly unusual properties and an improved understanding of structure-property relationships in compounds containing structurally different layers. A goal is to understand the dependence of physical properties on the identity, thickness, and the sequence of individual layers. A second goal is to understand the fundamental aspects of the synthesis approach that result in the preparation of stable products. Current and future technologies crucial to international competitiveness depend on being able to both prepare and characterize stable layered materials to obtain enhanced properties, which are not found in any of the individual components. Technical Abstract:This research extends a synthesis approach to create new, layered solids containing two or more structurally different constituents with atomically abrupt interfaces between them. Designed precursors enable kinetically stable heterostructures with designed nanoarchitectures to be prepared over large areas. The project goal is to understand the dependence of transport properties on nanoarchitecture in heterostructures containing electrically isolated two dimensional layers of transition metal dichalcogenides, bismuth chalcogenides and related ternary structures. Large band gap spacer layers of varying thickness electrically isolate the dichalcogenide monolayers and adjacent magnetic layers are used to perturb the monolayers. This research is timely, as recent discoveries promise advances in a variety of technologies including tunnelling transistors, flexible electronics, photodetectors, photovoltaics and light-emitting devices with unprecedented characteristics and/or unique functionalities. This research provides a broad technical background for graduate students in deposition technologies, thin film characterization techniques, and physical phenomena that occur in 2D heterostructures. This training enables them to thrive in careers in high tech industries, academia or national laboratories.
非技术摘要:材料研究中的一个重大挑战是制备具有设计性能的新型化合物。通过复杂的分层方案创建稳定的分层材料的能力提供了前所未有的能力来探索成分的结构、组成和物理性能之间的相互作用。这项研究产生了丰富的新材料集合,具有不同和非常不寻常的性质,并改进了对含有不同结构层的化合物的结构-性质关系的理解。目标是了解物理属性对各个层的身份、厚度和顺序的依赖关系。第二个目标是了解导致制备稳定产品的合成方法的基本方面。当前和未来的技术对国际竞争力至关重要,取决于能否制备和表征稳定的层状材料以获得增强的性能,这是任何单个部件都找不到的。技术摘要:这项研究扩展了一种合成方法,以创造包含两个或更多结构不同的组分的新的层状固体,它们之间具有原子突变的界面。设计的前驱体使具有设计的纳米结构的动力学稳定的异质结构能够在大范围内制备。该项目的目标是了解异质结构中纳米结构对输运性质的依赖,该异质结构包含电隔离的过渡金属二卤化物、硫化物铋和相关的三元结构的二维层。可变厚度的大带隙间隔层电隔离二碳化合物单分子层,并且使用相邻的磁性层来扰乱单分子层。这项研究是及时的,因为最近的发现有望在各种技术方面取得进展,包括隧道晶体管、柔性电子设备、光电探测器、光伏和具有前所未有的特性和/或独特功能的发光设备。这项研究为研究生在沉积技术、薄膜表征技术以及2D异质结构中出现的物理现象方面提供了广泛的技术背景。这种培训使他们能够在高科技行业、学术界或国家实验室的职业生涯中茁壮成长。

项目成果

期刊论文数量(27)
专著数量(0)
科研奖励数量(0)
会议论文数量(0)
专利数量(0)
Strong Non-Epitaxial Interactions: Crystallographically Aligned PbSe on VSe 2
强非外延相互作用:VSe 2 上晶体排列的 PbSe
  • DOI:
    10.1002/pssa.201800896
  • 发表时间:
    2019
  • 期刊:
  • 影响因子:
    0
  • 作者:
    Cordova, Dmitri L.;Kam, Taryn M.;Fender, Shannon S.;Tsai, Yu Hsin;Johnson, David C.
  • 通讯作者:
    Johnson, David C.
Structural Changes as a Function of Thickness in [(SnSe) 1+δ ] m TiSe 2 Heterostructures
[(SnSe) 1 δ ] m TiSe 2 异质结构中的结构变化随厚度变化
  • DOI:
    10.1021/acsnano.7b07506
  • 发表时间:
    2018
  • 期刊:
  • 影响因子:
    17.1
  • 作者:
    Hamann, Danielle M.;Lygo, Alexander C.;Esters, Marco;Merrill, Devin R.;Ditto, Jeffrey;Sutherland, Duncan R.;Bauers, Sage R.;Johnson, David C.
  • 通讯作者:
    Johnson, David C.
Ultralow shear modulus of incommensurate [SnSe]n[MoSe2]n layers synthesized by the method of modulated elemental reactants
调制元素反应物法合成的不相称[SnSe]n[MoSe2]n层的超低剪切模量
  • DOI:
    10.1103/physrevmaterials.3.043607
  • 发表时间:
    2019
  • 期刊:
  • 影响因子:
    3.4
  • 作者:
    Li, Dongyao;Schleife, André;Cahill, David G.;Mitchson, Gavin;Johnson, David C.
  • 通讯作者:
    Johnson, David C.
Electronic structure of designed [(SnSe)1+δ]m[TiSe2]2 heterostructure thin films with tunable layering sequence
具有可调分层顺序的[(SnSe)1 δ]m[TiSe2]2异质结构薄膜的电子结构
  • DOI:
    10.1557/jmr.2019.128
  • 发表时间:
    2019
  • 期刊:
  • 影响因子:
    2.7
  • 作者:
    Göhler, Fabian;Hamann, Danielle M.;Rösch, Niels;Wolff, Susanne;Logan, Jacob T.;Fischer, Robert;Speck, Florian;Johnson, David C.;Seyller, Thomas
  • 通讯作者:
    Seyller, Thomas
Sub-Monolayer Accuracy in Determining the Number of Atoms per Unit Area in Ultrathin Films Using X-ray Fluorescence
  • DOI:
    10.1021/acs.chemmater.8b02591
  • 发表时间:
    2018-09-25
  • 期刊:
  • 影响因子:
    8.6
  • 作者:
    Hamann, Danielle M.;Bardgett, Dylan;Johnson, David C.
  • 通讯作者:
    Johnson, David C.
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David Johnson其他文献

The effect of caffeine and choline on short term memory
咖啡因和胆碱对短期记忆的影响
  • DOI:
  • 发表时间:
    2011
  • 期刊:
  • 影响因子:
    0
  • 作者:
    Natasha Nagrecha;Vincent Giannetti;P. Witt‐Enderby;Jamie L. McConaha;Amit Patel;David Johnson
  • 通讯作者:
    David Johnson
Identification of Molecular Markers Associated with Verticillium Wilt Resistance in Alfalfa (Medicago Sativa L.) Using High-Resolution Melting
使用高分辨率熔化鉴定与苜蓿 (Medicago Sativa L.) 黄萎病抗性相关的分子标记
  • DOI:
  • 发表时间:
    2014
  • 期刊:
  • 影响因子:
    3.7
  • 作者:
    Tie;Long;P. McCord;David J. Miller;S. Bhamidimarri;David Johnson;M. Monteros;J. Ho;P. Reisen;D. Samac
  • 通讯作者:
    D. Samac
Ambiguity in Performance Pay: An Online Experiment
绩效工资的模糊性:在线实验
Analysis of 10 metabolites of polymethoxyflavones with high sensitivity by electrochemical detection in high-performance liquid chromatography
高效液相色谱电化学检测高灵敏度分析多甲氧基黄酮10种代谢物
  • DOI:
    10.1021/jf505545x
  • 发表时间:
    2015
  • 期刊:
  • 影响因子:
    6.1
  • 作者:
    Jinkai Zheng;Jinfeng Bi;David Johnson;Yue Sun;Mingyue Song;Peiju Qiu;Ping Dong;Eric Decker;Hang Xiao
  • 通讯作者:
    Hang Xiao
Disruption of NOX2-dependent Oxidative Injury with a Targeted Gene-Therapy Approach Prevents Atrial Fibrillation in a Canine Model
用靶向基因治疗方法破坏 NOX2 依赖性氧化损伤可预防犬模型中的心房颤动
  • DOI:
    10.1101/765008
  • 发表时间:
    2019
  • 期刊:
  • 影响因子:
    0
  • 作者:
    S. Yoo;Anna Pfenniger;Jacob Hoffman;Wenwei Zhang;J. Ng;Amy Burrell;David Johnson;Georg Gussak;Trent Waugh;Suzanne Bull;Brandon C. Benefield;B. Knight;R. Passman;J. Wasserstrom;G. Aistrup;R. Arora
  • 通讯作者:
    R. Arora

David Johnson的其他文献

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{{ truncateString('David Johnson', 18)}}的其他基金

CAREER: Risk-Based Methods for Robust, Adaptive, and Equitable Flood Risk Management in a Changing Climate
职业:在气候变化中实现稳健、适应性和公平的洪水风险管理的基于风险的方法
  • 批准号:
    2238060
  • 财政年份:
    2023
  • 资助金额:
    $ 45万
  • 项目类别:
    Standard Grant
European Partnering Award: Harnessing root-fungal symbioses for sustainable agri-ecosystems
欧洲合作奖:利用根真菌共生实现可持续农业生态系统
  • 批准号:
    BB/X018210/1
  • 财政年份:
    2023
  • 资助金额:
    $ 45万
  • 项目类别:
    Research Grant
Functioning of soil food webs in response to woodland expansion
土壤食物网的功能响应林地扩张
  • 批准号:
    NE/X011135/1
  • 财政年份:
    2023
  • 资助金额:
    $ 45万
  • 项目类别:
    Research Grant
Collaborative Research: Exploring thermionic multiple barrier heterostructures and thermoelectric energy conversion using 2D layered heterostructures
合作研究:利用二维层状异质结构探索热离子多重势垒异质结构和热电能量转换
  • 批准号:
    2323032
  • 财政年份:
    2023
  • 资助金额:
    $ 45万
  • 项目类别:
    Standard Grant
Short-circuiting the terrestrial phosphorus cycle: symbiotic control of organic phosphorus mineralisation and uptake
缩短陆地磷循环:有机磷矿化和吸收的共生控制
  • 批准号:
    NE/W000350/1
  • 财政年份:
    2022
  • 资助金额:
    $ 45万
  • 项目类别:
    Research Grant
Synthesis and Properties of Heterostructures Containing Magnetic 2d Layers Not Found As Bulk Compounds
含有未发现为本体化合物的磁性二维层的异质结构的合成和性能
  • 批准号:
    2219512
  • 财政年份:
    2022
  • 资助金额:
    $ 45万
  • 项目类别:
    Standard Grant
SAI-R: Reducing Natural Hazards Risks by Incorporating Community Impacts and Equity
SAI-R:通过纳入社区影响和公平来减少自然灾害风险
  • 批准号:
    2228559
  • 财政年份:
    2022
  • 资助金额:
    $ 45万
  • 项目类别:
    Standard Grant
21EJP SOIL: SymbiOtIc soLutions for HEalthy Agricultural Landscapes (SOIL HEAL)
21EJP SOIL:健康农业景观的共生解决方案(土壤修复)
  • 批准号:
    BB/X000729/1
  • 财政年份:
    2022
  • 资助金额:
    $ 45万
  • 项目类别:
    Research Grant
Maximising ecosystem services in urban environments (MEaSURE)
最大化城市环境中的生态系统服务(MEaSURE)
  • 批准号:
    NE/W003120/1
  • 财政年份:
    2021
  • 资助金额:
    $ 45万
  • 项目类别:
    Research Grant
Collaborative Research: Understanding Cross-plane and In-plane Transport in 2D Layered Heterostructures
合作研究:了解二维层状异质结构中的跨平面和面内传输
  • 批准号:
    1905185
  • 财政年份:
    2019
  • 资助金额:
    $ 45万
  • 项目类别:
    Standard Grant

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Synthesis, Structure and Photoluminescent Properties of Perovskite - Hybrid Glass Composites
钙钛矿-杂化玻璃复合材料的合成、结构及光致发光性能
  • 批准号:
    2748737
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    2022
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Use of De Novo Synthesis Approaches and Structure-guided Design to Optimize Therapeutic Properties of Streptothricin Class Antimicrobials
使用从头合成方法和结构引导设计来优化链丝菌素类抗菌药物的治疗特性
  • 批准号:
    10469007
  • 财政年份:
    2020
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    $ 45万
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Use of De Novo Synthesis Approaches and Structure-guided Design to Optimize Therapeutic Properties of Streptothricin Class Antimicrobials
使用从头合成方法和结构引导设计来优化链丝菌素类抗菌药物的治疗特性
  • 批准号:
    10269053
  • 财政年份:
    2020
  • 资助金额:
    $ 45万
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Use of De Novo Synthesis Approaches and Structure-guided Design to Optimize Therapeutic Properties of Streptothricin Class Antimicrobials
使用从头合成方法和结构引导设计来优化链丝菌素类抗菌药物的治疗特性
  • 批准号:
    10686110
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RUI: Exploring Synthesis, Tailoring Structure, Evaluating Properties, and Enabling Patterning of Surface-Anchored Framework Assemblies
RUI:探索表面锚定框架组件的合成、定制结构、评估属性和实现图案化
  • 批准号:
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Precise synthesis of architectural polymers with luminescent units at polymer connection points and evaluation of the correlation between structure and physical properties
在聚合物连接点处具有发光单元的建筑聚合物的精确合成以及结构与物理性能之间的相关性评估
  • 批准号:
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Synthesis, structure and properties of functionalized mesoporous hybrid materials
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Synthesis, structure and properties of responsive solid-state materials
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  • 批准号:
    RGPIN-2014-05534
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    2018
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    $ 45万
  • 项目类别:
    Discovery Grants Program - Individual
Synthesis, structure and properties of responsive solid-state materials
响应性固态材料的合成、结构与性能
  • 批准号:
    RGPIN-2014-05534
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    Discovery Grants Program - Individual
Synthesis and Properties of Chalcogenocarbonyl Complexes with a Half-Sandwiched Structure
半夹心结构硫属羰基配合物的合成及性能
  • 批准号:
    17K05817
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  • 项目类别:
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