Nonlinear optrical properties of the natural quantum-well materials

天然量子阱材料的非线性光学特性

基本信息

  • 批准号:
    04452101
  • 负责人:
  • 金额:
    $ 4.42万
  • 依托单位:
  • 依托单位国家:
    日本
  • 项目类别:
    Grant-in-Aid for General Scientific Research (B)
  • 财政年份:
    1992
  • 资助国家:
    日本
  • 起止时间:
    1992 至 1993
  • 项目状态:
    已结题

项目摘要

Linear and nonlinear optical properties of excitons in the natural quantum-well materials have been investigated and the following results have been obtained.1. Magnetooptical studyExcitons in (C_6H_<13>NH_3)_2PbI_4 and other related compounds are strongly localized Frenkel type excitons mainly composed of Pb^<2+> 6s 6p orbitals.2. Nonlinear spectroscopyA pump-prove experiment was paeformed on ((C_6H_<13>NH_3)_2PbI_4 using a ns pulse laser, and a strong absorption saturation up to 50 % was observed. This corresponds to chi^<(3)> - 10^<-4> esu. In a photoluminescence measurement, a strong "nonlinear" luminescence peak was observed. Unfortunately, its origin has not been understood.3. Degenerate four wave mixingchi^<(3)> spectra were measured by degenerate four wave mixing experiments on (C_6H_<13>NH_3)_2PbI_4 using a ns pulse laser. The obtained chi^<(3)> reaches 6 X 10^<-4> esu at room temperature and 2.4 X 10^<-3> esu at 77 K showing strong one-photon resonances to the absorption peaks. These chi^<(3)> values are much larger than that measured by THG, 10^<-9> esu.In order to investigate the origin of the lager chi^<(3)>, time-resolved pump-probe experiments are now underway.
研究了自然量子阱材料中激子的线性和非线性光学性质,得到了以下结果.磁光研究(C_6H_NH_3<13>)_2PbI_4及其它相关化合物中的激子是强定域的Frenkel型激子,主要由Pb^&lt;2+&gt; 6s 6p轨道组成.用纳秒脉冲激光对((C_6H_NH_3)_2PbI_4)进行了泵浦验证实验<13>,观察到了50%的强吸收饱和。这对应于chi^&lt;(3)&gt; - 10^<-4>esu。在光致发光测量中,观察到强的“非线性”发光峰。不幸的是,它的起源一直没有被理解。用纳秒脉冲激光对(C_6H_NH_3)_2PbI_4进行了简并四波混频实验,测量了简并四波混频χ ^&lt;3&gt;谱<13>。在室温和77 K下,x ^&lt;3&gt;分别达到6 × 10 ~(10)<-4>esu和2.4 × 10 ~(10)<-3>esu,表现出较强的单光子共振。这些chi^&lt;3&gt;值比THG测量的值大得多<-9>,为研究大chi^&lt;3&gt;的起源,时间分辨泵浦探测实验正在进行中。

项目成果

期刊论文数量(26)
专著数量(0)
科研奖励数量(0)
会议论文数量(0)
专利数量(0)
Y.Takeda: "“Third-Order Optical Nonlinearity of the Natural Quantum-Well Material(C_6H_<13>NH_3)_2PbI_4"" Submitted to Jpn.J.Appl.Phys.
Y.Takeda:“天然量子阱材料的三阶光学非线性(C_6H_<13>NH_3)_2PbI_4”提交给Jpn.J.Appl.Phys。
  • DOI:
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    0
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  • 通讯作者:
T.Kondo,C-Q.Xu and R.Ito: "Linear and Nonlinear Optical Properties of a Natural Quantum-Well Material (C_<10>H_<21>NH_3)_2PbI_4" Nonlinear Optics (Elsevier). 323-328 (1992)
T.Kondo、C-Q.Xu 和 R.Ito:“天然量子阱材料 (C_<10>H_<21>NH_3)_2PbI_4 的线性和非线性光学特性”非线性光学 (Elsevier)。
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    0
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  • 通讯作者:
T.Kataoka, T.Kondo, R.Ito, S.Sasaki, K.Uchida and N.Miura: ""Magneto-Optica Study on Excitonic Spectrum of (C_6H_<13>NH_3)_<2->PbI_4"" Phys.Rev.B47. 2010-2018 (1993)
T.Kataoka、T.Kondo、R.Ito、S.Sasaki、K.Uchida 和 N.Miura:“(C_6H_<13>NH_3)_<2->PbI_4 激子谱的磁光研究”物理
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  • 影响因子:
    0
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  • 通讯作者:
Y.Takeda, T.Kataoka, T.Kondo, T.Motohiro and R.Ito: ""Third-Order Optical Nonlinearity of the Natural Quantum-Well Material (C_6H_<13>NH_3)_2PbI_4"" Jpn.J.Appl.Phys.(Submitted to).
Y.Takeda、T.Kataoka、T.Kondo、T.Motohiro 和 R.Ito:“天然量子阱材料 (C_6H_<13>NH_3)_2PbI_4 的三阶光学非线性”Jpn.J.Appl。
  • DOI:
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  • 期刊:
  • 影响因子:
    0
  • 作者:
  • 通讯作者:
T.Kataoka: "“Magneto-Optical Study on the Excitonic Spectrum of(C_6H_<13>-NH_3)_2PbI_4"" Physica B. 184. 132-136 (1993)
T. Kataoka:“(C_6H_<13>-NH_3)_2PbI_4 激子谱的磁光研究” Physica B. 184. 132-136 (1993)
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    0
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ITO Ryoichi其他文献

ITO Ryoichi的其他文献

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{{ truncateString('ITO Ryoichi', 18)}}的其他基金

Quadratic Nonlipear Optical Properties Studied by Reflected Second-Harmonic Ellipsometry
反射二次谐波椭圆光度法研究二次非唇形光学特性
  • 批准号:
    11305010
  • 财政年份:
    1999
  • 资助金额:
    $ 4.42万
  • 项目类别:
    Grant-in-Aid for Scientific Research (A)
Domain-Inversion Epitaxy and Its Application to Wavelength Conversion Devices
畴反转外延及其在波长转换器件中的应用
  • 批准号:
    08405002
  • 财政年份:
    1996
  • 资助金额:
    $ 4.42万
  • 项目类别:
    Grant-in-Aid for Scientific Research (A)
Research on Frequency Conversion in Nonlinear Optical Heterostructures
非线性光学异质结构频率转换研究
  • 批准号:
    06452126
  • 财政年份:
    1994
  • 资助金额:
    $ 4.42万
  • 项目类别:
    Grant-in-Aid for General Scientific Research (B)
Davelopment of Nonlinear Optical Frequency-Conversion Micro Devices Using Micro-Fabrication Technique for Organic Crystals
利用有机晶体微加工技术开发非线性光学变频微型器件
  • 批准号:
    04555012
  • 财政年份:
    1992
  • 资助金额:
    $ 4.42万
  • 项目类别:
    Grant-in-Aid for Developmental Scientific Research (B)
Optical Properties of Layered Perovskite Materials with Natural Quantum-Well Structure
具有天然量子阱结构的层状钙钛矿材料的光学性质
  • 批准号:
    02452072
  • 财政年份:
    1990
  • 资助金额:
    $ 4.42万
  • 项目类别:
    Grant-in-Aid for General Scientific Research (B)
Development of Nonlinear Optical Waveguiding Devices for Second-Harmonic Generation of Laser Diode Light
用于激光二极管光二次谐波产生的非线性光波导器件的开发
  • 批准号:
    63850012
  • 财政年份:
    1988
  • 资助金额:
    $ 4.42万
  • 项目类别:
    Grant-in-Aid for Developmental Scientific Research (B).
Development of Highly Efficient, Visible Coherent Light Sources Using Semiconductor Lasers and Organic Nomlinear Optical Materials
使用半导体激光器和有机非线性光学材料开发高效可见相干光源
  • 批准号:
    61460072
  • 财政年份:
    1986
  • 资助金额:
    $ 4.42万
  • 项目类别:
    Grant-in-Aid for General Scientific Research (B)

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研究超晶格中的声子散射,以设计高效的多量子阱热载流子太阳能电池
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