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Pressure induced Novel quantum phenomena in Q2D Mott transition system Ca_2RuO_4

Q2D莫特跃迁体系Ca_2RuO_4中压力诱导的新量子现象

基本信息

批准号：
17540328
负责人：
NAKAMURA Fumihiko
金额：
$ 2.24万
依托单位：
HIROSHIMA UNIVERSITY
依托单位国家：
日本
项目类别：
Grant-in-Aid for Scientific Research (C)
财政年份：
2005
资助国家：
日本
起止时间：
2005 至 2006
项目状态：
已结题

来源：
https://kaken.nii.ac.jp/en/grant/KAKENHI-PROJECT-17540328/
关键词：
strongly correlated electron pressure effect Ru oxides Mott transition system Quantum Critical Point Giant magnetoresistance Itinerant ferromagnetism

项目摘要

To explore novel quantum phenomena such as unconventional superconductivity, itinerant magnetism, and large magnetoresistance effect is one of the most important and interesting subjects in condensed matter physics. Much attention has been paid for a Mott transition system in single-layered ruthenate oxides. This is because the materials display versatile quantum phenomena, ranging from an antiferromagnetic (AF) Mott insulator to a ferromagnetic (FM) metal, as well as the superconductor. In particular, the pressure phase diagram is quite unique and different from that of the doped system. In this project, we feature two interesting phenomena as follows :1. Anisotropic giant magnetoresistance effect in the vicinity of Mott transitionWe have observed an anisotropic and giant magnetoresistance (MR) of a 4d-electron system Ca_2RuO_4 in the vicinity of a pressure induced Mott transition. At〜2GPa, the MR effect at 10T reaches〜-80% at〜T_c for longitudinal and 〜+80% at low temperatures for the transverse effects. The negative MR is interpreted as a reduction of a FM spin fluctuation at T_c. In contrast, the observed large positive effect is rare and likely due to metal-nonmetal transition induced by applying fields along the c axis.2. Itinerant ferromagnetism in the quasi-2D metallic stateWe reveal that pressurisation to Ca_2RuO_4 transforms it from a Mott insulator with an AF ground state to a quasi-2D metal with a FM ground state. This ferromagnetism has been observed in the metallic phase, and then contains features of an itinerant FM. Firstly, M_<rem>〜35μ_B is quite smaller than the saturated moment of 2μ_B of localised Ru^<4+> ion. Secondly, a ratio of p_<eff> / M_<rem>〜5 is much larger than 1 of localized spins systems. Lastly, M is not easily saturated with H. In particular, the magnetisation process at low temperatures exhibits good linearity in an Arrott plot (M_<rem>^2 versus H/M plot). These FM natures are comparable to typical itinerant ferromagnet of MnSi.

探索非常规超导、巡回磁性、大磁阻效应等新颖的量子现象是凝聚态物理中最重要和最有趣的课题之一。单层钌酸盐氧化物中的莫特转变体系受到了很多关注。这是因为这些材料表现出多种量子现象，从反铁磁 (AF) 莫特绝缘体到铁磁 (FM) 金属以及超导体。特别是，压力相图非常独特，与掺杂系统的压力相图不同。在这个项目中，我们有两个有趣的现象：1。莫特跃迁附近的各向异性巨磁阻效应我们在压力引起的莫特跃迁附近观察到了 4d 电子系统 Ca_2RuO_4 的各向异性巨磁阻（MR）。在~2GPa下，10T下的MR效应在~T_c下纵向达到~-80%，在低温下横向效应达到~+80%。负 MR 被解释为 T_c 处 FM 自旋波动的减少。相反，观察到的大的积极效应是罕见的，可能是由于沿c轴施加场引起的金属-非金属转变所致。2．准二维金属态的巡回铁磁性我们揭示了对 Ca_2RuO_4 的加压会将其从具有 AF 基态的莫特绝缘体转变为具有 FM 基态的准二维金属。这种铁磁性已在金属相中观察到，并且包含流动 FM 的特征。首先，M_<rem>〜35μ_B远小于局域Ru^<4+>离子的2μ_B的饱和矩。其次，局域自旋系统的 p_<eff> / M_<rem>〜5 的比率远大于 1。最后，M 不容易被 H 饱和。特别是，低温下的磁化过程在 Arrott 图（M_<rem>^2 与 H/M 图）中表现出良好的线性。这些 FM 性质与典型的 MnSi 流动铁磁体相当。

项目成果

期刊论文数量（18）

专著数量（0）

科研奖励数量（0）

会议论文数量（0）

专利数量（0）

Pressure-induced Mott transition and related novel quantum phenomena in Ca2Ru04

Ca2Ru04 中压力诱导的莫特跃迁及相关新量子现象

DOI：
发表时间：
2007
期刊：
J. Phys. Soc. Jpn. 76 (in press)
影响因子：
0
作者：
F.Honda;N.Metoki;K.Kaneko;S.Jonen;E.Yamamoto;D.Aoki;Y.Homma;Y.Haga;Y.Shiokawa;Y.Onuki;Koji Ueda et al.;Fumihiko Nakamura
通讯作者：
Fumihiko Nakamura

Magnetic heat transport in RcCuO4 (R=La, Pr, Nd, Sm, Eu, and Gd)

RcCuO4 中的磁热传输（R=La、Pr、Nd、Sm、Eu 和 Gd）

DOI：
发表时间：
2006
期刊：
Physical Review B 73
影响因子：
0
作者：
K.Berggold;F.Nakanura;et al.
通讯作者：
et al.

Development of a piston-cylinder pressure cell using nonmagnetic and high-yield strength alloys for a SQUID magnetometer

使用非磁性高屈服强度合金开发用于 SQUID 磁力计的活塞缸压力传感器

DOI：
发表时间：
2007
期刊：
J. Phys. Soc. Jpn. 76 (in press)
影响因子：
0
作者：
R.NAKAI;F.NAKAMURA;T.SUZUKI
通讯作者：
T.SUZUKI

Evidence for suppressed screening on the surface of high temperature La2-xSrxCuO4 and Nd2-xCexCuO4 superconductors

高温 La2-xSrxCuO4 和 Nd2-xCexCuO4 超导体表面抑制屏蔽的证据

DOI：
发表时间：
2005
期刊：
Phys Rev. Lett. 95
影响因子：
0
作者：
M. Taguchi;A. Chainani;K. Horiba;Y. Takata;S. Shin;T. Yokoya;E. Ikenaga;K. Kobayashi;T. Mochiku;K. Hirata;J. Hori;T. Suzuki
通讯作者：
T. Suzuki

Pressure-induced Mott transition and related novel quantum phenomena in Ca_2RuO_4

Ca_2RuO_4 中压力诱导的莫特跃迁及相关新量子现象