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Chemical Synthesis of Pheromones of Insects, Flagellates and Mammals.

Chemical Synthesis of Pheromones of Insects, Flagellates and Mammals.
昆虫、鞭毛虫和哺乳动物信息素的化学合成。
批准号：
09680576
负责人：
MORI Kenji
金额：
$2.05万
依托单位：
Science University of Tokyo
依托单位国家：
日本
项目类别：
Grant-in-Aid for Scientific Research (C)
财政年份：
1997
资助国家：
日本
项目状态：
已结题
起止时间：
1997 至 1998
来源：
https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-09680576/
关键词：
pheromonesoptically active compoundscymmetric synthesis

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中文摘要
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英文摘要
1. Lurlenic acid, the female-produced pheromone of the green flagellate Chlamydomonas allensworthii, and its analogues were synthesized. Structural requirements for the expression of the pheromone activity are the sugar-part, the phenol part and the unsaturated side-chain with a polar group at its end.2. Bark beetle pheromones such as endo-isobrevicomin, exo-isobrevicomin, bicolorin, frontalin etc. were synthesized.3. Stegobiol and stegobinone, the drugstore beetle pheromone, were synthesized.4. Stigmolone, the pheromone to induce the fruiting body formation of a myxobacterium Stigmatella aurantiaca, was synthesized. The natural pheromone is a racemate.5. The racemate of the male-produced sex pheromone of the sandfly Lutzomyia longipalpis, (*)-3-methyl-alpha-himachalene and (*)-9-methylgermacrene-B, were synthesized to establish the gross structures of the pheromone components.6. The enantiomers of 2-sec-butyl-4, 5-dihydrothiazole and (lR, 5S, 7R)-3, 4-dehydro-exo-brevicomin, the pheromone components of the house mouse Mus musculus, were synthesized.
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会议论文
S.Takanashi, K.Mori: "Synthesis of the Analogues of Lurlent Acid with modification in the Side-chain or in the Aromatic Nucleus : Summary of the Structure-Activity Relationships" Eurupeam Journal of Organic Chemistry. 43-55 (1998)
S.Takanashi、K.Mori：“侧链或芳香核修饰的 Lurlent 酸类似物的合成：结构-活性关系总结”Europeam 有机化学杂志。
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通讯作者：
S.Muto,Y.Nishimura,K.Mori: "Synthesis of Germacrene-B and Its Extension to the Synthesis of (±)-9-Methylgermacrene-B, the Racemate of the Male-produced Sex Pheromone of the Sandfly" European Journal of Organic Chemistry. 印刷中. (1999)
S.Muto、Y.Nishimura、K.Mori：“Germacrene-B 的合成及其对 (±)-9-Mmethylgermacrene-B（白蛉雄性产生的性信息素的外消旋体）合成的延伸”欧洲期刊有机化学出版（1999）。
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S.Takanashi, K.Mori: "Synthesis of the Analogues of Lurlemic Acid with a modified Sugar pant : Chlamydomonas responds only to the D-xyluside" Liebigs Annalen. 1081-1084 (1997)
S.Takanashi、K.Mori：“用改良糖裤合成 Lurlemic Acid 类似物：衣藻仅对 D-木糖苷有反应”Liebigs Annalen。
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通讯作者：
S.Sano, K.Mori: "Synthesis of (1R^*, 3R^*, 7R^*)-3-Methyl-α-himachalene, the Racemate of the Male-produced Sex Pheromone of the Sandfly" European Journal of Organic Chemistry. (印刷中). (1999)
S.Sano, K.Mori：“白蛉雄性产生的性信息素的外消旋体 (1R^*, 3R^*, 7R^*)-3-甲基-α-himachalene 的合成”《欧洲有机杂志》化学（正在出版）（1999）。
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