Two dimensional atomic crystals under strain

应变下的二维原子晶体

• 批准号: 1808491
• 负责人: Xu Du
• 金额: $ 45.48万
• 依托单位: SUNY at Stony Brook
• 依托单位国家: 美国
• 项目类别: Standard Grant
• 财政年份: 2018
• 资助国家: 美国
• 起止时间: 2018-08-15 至 2023-07-31
• 项目状态: 已结题
• 来源: https://www.nsf.gov/awardsearch/showAward?AWD_ID=1808491&HistoricalAwards=false
• 关键词: Two; dimensional; atomic; crystals; under

Non-Technical Description:Two-dimensional atomic crystals, the building blocks for layered materials, have promising electrical/optical properties that are strongly affected by their structures. Formed through strong chemical bonds, these materials can be atomically thin yet act like a crystal with the ability to bend. It is both interesting and important to understand how the crystal deformation (strain) may modify their electronic and charge transport properties. Based on such understanding, lattice deformation may be used for better electronic properties and to create novel material systems for the study of low dimensional physics. This project studies the impact of strain on the electronic and charge transport properties of two-dimensional atomic crystals in their nanoelectromechanical devices, where strain can be independently tuned and accurately characterized. This project addresses some of the key scientific and technological issues in a highly active research area. It also provides graduate students with research experience both in the PI's Stony Brook laboratory and in national laboratory settings. Undergraduate students drawn from the diverse student body of Stony Brook University and high school students from the greater New York region will be brought in to play active roles in the research. To widen the general public interest in sciences, the research team will broadcast original videos on student research in the lab, and introductions to basic experimental research techniques.Technical Description:Two-dimensional atomic crystals are formed through strong chemical bonds which render them flexible and stretchable in nature. As a result, lattice deformation may be utilized to achieve more favorable electronic properties and to create novel material systems for the study of low dimensional physics. The project is developing a nanoelectromechanical resonator device scheme with large strain tunability and transport measurement capability, through which both the mechanical and charge transport properties are studied and correlated. This approach is applied to two-dimensional atomic crystals including (but not limited to) single- and bi-layer graphene, phosphorene, and ZrTe5. The research team focuses on the impact of mechanical deformation (including uniaxial, shear and triaxial strains) on charge carrier scattering, valley polarization, band structure tuning, and topological transitions in these two-dimensional materials. The project advances the understanding in the fundamental physical properties of novel two dimensional materials and in modulating their electronic properties to study novel two-dimensional physics. Modification of lattice structure and/or symmetry can effectively create new artificial material systems which allow the study of novel physical phenomena inaccessible in conventional materials. This proposal, which focuses mainly on charge transport studies, directly addresses fabrication and measurement of the electronic devices. Hence, it further advances the concept of strain-tunable electronics beyond the previous efforts which are mainly based on optical and local probe studies.This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.

非技术描述：二维原子晶体是层状材料的构建块，具有受其结构强烈影响的有前途的电学/光学特性。通过强化学键形成，这些材料可以像原子一样薄，但却像晶体一样具有弯曲的能力。了解晶体变形（应变）如何改变其电子和电荷输运性质既有趣又重要。基于这样的理解，晶格变形可以用于更好的电子性质，并创建用于低维物理研究的新材料系统。该项目研究了应变对纳米机电设备中二维原子晶体的电子和电荷传输特性的影响，其中应变可以独立调整和准确表征。该项目涉及一个高度活跃的研究领域的一些关键科学和技术问题。它还为研究生提供了在PI的斯托尼布鲁克实验室和国家实验室环境中的研究经验。来自斯托尼布鲁克大学多元化学生团体的本科生和来自大纽约地区的高中生将在研究中发挥积极作用。为了提高公众对科学的兴趣，研究团队将播放学生在实验室进行研究的原创视频，并介绍基本的实验研究技术。技术说明：二维原子晶体是通过强化学键形成的，使其具有柔性和可拉伸性。因此，晶格变形可以用来实现更有利的电子性质，并创建新的材料系统的低维物理的研究。该项目正在开发一种具有大应变可调谐性和输运测量能力的纳米机电谐振器器件方案，通过该方案研究和关联机械和电荷输运性质。这种方法适用于二维原子晶体，包括（但不限于）单层和双层石墨烯，磷烯和ZrTe 5。该研究小组专注于机械变形（包括单轴，剪切和三轴应变）对这些二维材料中的电荷载流子散射，谷极化，能带结构调谐和拓扑转变的影响。该项目推进了对新型二维材料基本物理性质的理解，并调节其电子性质以研究新型二维物理。晶格结构和/或对称性的修改可以有效地创建新的人工材料系统，其允许研究在常规材料中无法实现的新物理现象。该提案主要侧重于电荷传输研究，直接涉及电子器件的制造和测量。该奖项反映了NSF的法定使命，并通过使用基金会的知识价值和更广泛的影响审查标准进行评估，被认为值得支持。

项目成果

Infrared nano-imaging of Dirac magnetoexcitons in graphene

• DOI: 10.1038/s41565-023-01488-y
• 发表时间: 2023-08-21
• 期刊: NATURE NANOTECHNOLOGY
• 影响因子: 38.3
• 作者: Dapolito, Michael;Tsuneto, Makoto;Liu, Mengkun
• 通讯作者: Liu, Mengkun

Contact transparency in mechanically assembled 2D material devices

• DOI: 10.1088/2515-7639/ab1863
• 发表时间: 2019-06
• 期刊: Journal of Physics: Materials
• 作者: S. Mills;N. Mizuno;Peng Wang;J. Lyu;Kenji Watanabe;T. Taniguchi;F. Camino;Liyuan Zhang;Xu Du

Bandgap opening in MoTe2 thin flakes induced by surface oxidation

• DOI: 10.1007/s11467-020-0952-x
• 发表时间: 2020-03-05
• 期刊: FRONTIERS OF PHYSICS
• 影响因子: 7.5
• 作者: Gan, Yuan;Liang, Jiyuan;Zhang, Liyuan
• 通讯作者: Zhang, Liyuan